Photocatalytic Activity of Nonprecious Metal WSe2/g-C3N4 Composite Under Visible Light Irradiation

被引:7
作者
Wang, Jieqiong [1 ,2 ]
Yang, Jie [1 ]
Fang, Jian [1 ]
Li, Yuhang [1 ]
Zhang, Hongyuan [1 ]
Zhao, Zhenbo [1 ]
Ao, Yuhui [1 ]
机构
[1] Changchun Univ Technol, Sch Chem & Life Sci, Changchun 130012, Jilin, Peoples R China
[2] Changchun Univ Technol, Jilin Prov Key Lab Carbon Fiber Dev & Applicat, Changchun 130012, Jilin, Peoples R China
关键词
g-C3N4; WSe2; hydrothermal method; photocatalytic degradation; methyl orange; GRAPHITIC CARBON NITRIDE; HYDROGEN-EVOLUTION; ORGANIC-DYES; RHODAMINE-B; DEGRADATION; G-C3N4; NANOSHEETS; COCATALYST; GRAPHENE; WSE2;
D O I
10.1142/S1793292020500423
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
The WSe2/g-C3N4 (graphite carbon nitride) composite with photocatalytic properties was synthesized using a hydrothermal method. This synthesis pathway can be characterized by being simple, inexpensive and nonpolluting, integrating the concept of green chemistry. The WSe2/g-C3N4 composite could effectively degrade methyl orange solution under visible light irradiation. The decolorization experiment of methyl orange solution shows that the degradation rate of the 30 wt.% WSe2/g-C3N4 composite can reach 98.7% after 100 min of illumination, while the degradation rate of pure g-C3N4 was only 87.6% under the same conditions. This can be attributed to the fact that the combination of WSe2 and g-C3N4 nanosheets can increase the number of active binding sites, increasing the rate of charge separation and transport ability, decreasing the recombination rate of the photogenerated electron-hole pairs. Therefore, the WSe2/g-C3N4 composite will have potential development as a new material with low cost, easy synthesis and excellent performance in photocatalytic degradation of water pollution.
引用
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页数:12
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