Preparation of core-shell structured CoFe2O4 incorporated Ag3PO4 nanocomposites for photocatalytic degradation of organic dyes

被引:72
作者
Gan, Lu [1 ]
Xu, Lijie [2 ]
Qian, Kun [3 ]
机构
[1] Nanjing Forestry Univ, Coll Mat Sci & Engn, Nanjing 210037, Jiangsu, Peoples R China
[2] Nanjing Forestry Univ, Coll Biol & Environm, Nanjing 210037, Jiangsu, Peoples R China
[3] China Cleaner Prod Ctr Light Ind, Beijing 100012, Peoples R China
关键词
Ag3PO4-CoFe2O4; nanocomposite; Photocatalysis; Dye degradation; Magnetically separable; HIGHLY EFFICIENT; ENHANCED PHOTODEGRADATION; COMPOSITE; NANOPARTICLES; PERFORMANCE; STABILITY; AG;
D O I
10.1016/j.matdes.2016.07.043
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The core-shell structured CoFe2O4 incorporated Ag3PO4 nanocomposites were prepared through a precipitation approach. The structure of the prepared nanocomposites was investigated and the photocatalytic activity of the Ag3PO4-CoFe2O4 nanocomposites was studied through degrading methylene blue and rhodamine B dyes. The results showed that the CoFe2O4 nanoparticles were incorporated within the Ag3PO4 particles with a core-shell structure, narrowing the band gap of the Ag3PO4 at the same time. Compared with pure Ag3PO4, the Ag3PO4-CoFe2O4 nanocomposites had higher degradation efficiency to the dyes under the irradiation of the tungsten halogen lamp light. Moreover, due to the existence of the CoFe2O4, the Ag3PO4-CoFe2O4 nanocomposites were magnetically separable. The separated Ag3PO4-CoFe2O4 nanocomposites showed promising recycling stability for the photocatalysis degradation of the dyes. This study provides a novel nanocomposite which could photocatalytically degrade organic pollutants in wastewater without introducing secondary pollutant into the system. (C) 2016 Elsevier Ltd. All rights reserved.
引用
收藏
页码:354 / 360
页数:7
相关论文
共 38 条
[1]   WO3 nanorods/graphene nanocomposites for high-efficiency visible-light-driven photocatalysis and NO2 gas sensing [J].
An, Xiaoqiang ;
Yu, Jimmy C. ;
Wang, Yu ;
Hu, Yongming ;
Yu, Xuelian ;
Zhang, Guangjin .
JOURNAL OF MATERIALS CHEMISTRY, 2012, 22 (17) :8525-8531
[2]  
[Anonymous], RSC ADV
[3]   Graphene and TiO2 co-modified flower-like Bi2O2CO3. A novel multi-heterojunction photocatalyst with enhanced photocatalytic activity [J].
Ao, Yanhui ;
Xu, Liya ;
Wang, Peifang ;
Wang, Chao ;
Hou, Jun ;
Qian, Jin ;
Li, Yi .
APPLIED SURFACE SCIENCE, 2015, 355 :411-418
[4]   Preparation of graphene oxide-Ag3PO4 composite photocatalyst with high visible light photocatalytic activity [J].
Ao, Yanhui ;
Wang, Peifang ;
Wang, Chao ;
Hou, Jun ;
Qian, Jin .
APPLIED SURFACE SCIENCE, 2013, 271 :265-270
[5]   Efficient visible light photocatalysis of Bi4TaO8Cl nanoparticles synthesized by solution combustion technique [J].
Bhat, Swetha S. M. ;
Sundaram, Nalini G. .
RSC ADVANCES, 2013, 3 (34) :14371-14378
[6]   Ferromagnetism in lead graphite-pencils and magnetic composite with CoFe2O4 particles [J].
Bhowmik, R. N. .
COMPOSITES PART B-ENGINEERING, 2012, 43 (02) :503-509
[7]   Facet Effect of Single-Crystalline Ag3PO4 Sub-microcrystals on Photocatalytic Properties [J].
Bi, Yingpu ;
Ouyang, Shuxin ;
Umezawa, Naoto ;
Cao, Junyu ;
Ye, Jinhua .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2011, 133 (17) :6490-6492
[8]   Efficient synthesis of sunlight-driven ZnO-based heterogeneous photocatalysts [J].
Chang, Xueting ;
Li, Zhongliang ;
Zhai, Xinxin ;
Sun, Shibin ;
Gu, Danxia ;
Dong, Lihua ;
Yin, Yansheng ;
Zhu, Yanqiu .
MATERIALS & DESIGN, 2016, 98 :324-332
[9]   Novel Magnetically Separable Reduced Graphene Oxide (RGO)/ZnFe2O4/Ag3PO4 Nanocomposites for Enhanced Photocatalytic Performance toward 2,4-Dichlorophenol under Visible Light [J].
Chen, Xiaojuan ;
Dai, Youzhi ;
Guo, Jing ;
Liu, Tanhua ;
Wang, Xingyan .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2016, 55 (03) :568-578
[10]   High-Efficiency Visible-Light-Driven Ag3PO4/AgI Photocatalysts: Z-Scheme Photocatalytic Mechanism for Their Enhanced Photocatalytic Activity [J].
Chen, Zhihong ;
Wang, Weilin ;
Zhang, Zhengguo ;
Fang, Xiaoming .
JOURNAL OF PHYSICAL CHEMISTRY C, 2013, 117 (38) :19346-19352