Simultaneous biogas purification and CO2 capture by vacuum swing adsorption using zeolite NaUSY

被引:82
作者
Jiang, Yangyang [1 ]
Ling, Jianghua [2 ]
Xiao, Penny [3 ]
He, Yingdian [3 ]
Zhao, Qinghu [3 ]
Chu, Zheng [1 ]
Liu, Yingshu [4 ]
Li, Ziyi [4 ]
Webley, Paul A. [3 ]
机构
[1] Nanjing Chem Ind Grp, Sinopec Grp, Res Inst, Nanjing 210048, Jiangsu, Peoples R China
[2] Liaoning Shihua Univ, Fushun 113001, Peoples R China
[3] Univ Melbourne, Dept Chem Engn, Melbourne, Vic 3010, Australia
[4] Univ Sci & Technol Beijing, Sch Energy & Environm Engn, Beijing 100083, Peoples R China
关键词
Biogas purification; Zeolites; Activated carbon; Vacuum swing adsorption; ACTIVATED CARBON; FLUE-GAS; N-2; CH4; PRESSURE; SEPARATION; DIOXIDE; EQUILIBRIA; ADSORBENTS; SIMULATION;
D O I
10.1016/j.cej.2017.11.090
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In this study we report on a vacuum swing adsorption process and adsorbent which allows simultaneous production of high purity methane and high purity carbon dioxide from a biogas feedstock. This is a departure from conventional biogas purification processes which focus on production of high purity methane while venting the lower purity methane/carbon dioxide stream. Using NaUSY as the adsorbent, and based on experimental and simulation data, we are able to produce product purities of 98% CH4 and 95% CO2 in the two product streams, respectively, for an energy consumption of 0.23 GJ/tCO(2) from a feed containing 50/50% CH4/CO2.
引用
收藏
页码:2593 / 2602
页数:10
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