An experimental study of hydrogen autoignition in a turbulent co-flow of heated air

The autoignition behaviour of hydrogen in a turbulent co-flow of heated air at atmospheric pressures was examined experimentally. Turbulent flows of air, with temperatures up to 10 15 K and velocities up to 35 m/s, were set up in an optically accessible tube of circular cross-section. The fuel, pure or diluted with nitrogen, was continuously injected along the centreline of the tube, with velocities equal to or larger than those of the air, and temperatures that were lower. The fuel mixing patterns hence obtained were akin to diffusion from a point source or to an axisymmetric jet within a co-flow. For a relatively wide range of temperatures and velocities, a statistically steady condition of randomly occurring autoignition kernels was observed, whose axial location was measured by hydroxyl radical chemiluminescence. The probability density function of autoignition location was sharp enough to allow the accurate determination of a minimum autoignition length and smooth enough to allow the mean and variance to be calculated. It was found that both autoignition lengths increased with the air velocity and decreased with the air temperature, as expected. An estimate of the residence time up to autoignition showed that the autoignition delay times increased with the air velocity for the same temperature, suggesting a delaying effect of the turbulence on autoignition. The connection between these findings and previous experimental and direct numerical simulation studies is discussed. (c) 2004 The Combustion Institute. Published by Elsevier Inc. All rights reserved.