Formation of NOx from Air and N2/O2 Mixtures Using a Nonthermal Microwave Plasma System

被引:41
作者
Kim, Taesoo [1 ]
Song, Soonho [2 ]
Kim, Joongsoo [3 ]
Iwasaki, Ryuichi [4 ]
机构
[1] Yonsei Univ, Grad Sch, Dept Mech Engn, Seoul 120749, South Korea
[2] Yonsei Univ, Dept Mech Engn, Seoul 120749, South Korea
[3] Amarante Technol Inc, Santa Clara, CA 95054 USA
[4] Noritsu Koki Co Ltd, Plasma Business Div, Wakayama 6408550, Japan
关键词
BARRIER DISCHARGE; NITROGEN-OXIDES; GAS; REDUCTION; SPARK; O-3; GENERATION; HYDROGEN; ENERGY; OZONE;
D O I
10.1143/JJAP.49.126201
中图分类号
O59 [应用物理学];
学科分类号
摘要
We present an experimental study of NOx (NO and NO2) formation from air and N-2/O-2/NOx mixtures using a nonthermal microwave plasma device. The tests were performed considering the energy consumed to generate plasma gas and the flow rate of air. The results demonstrated that NOx production was proportional to input power and the inverse of air flow rate. In the experiments that used N-2 and O-2 mixtures instead of air, the maximum NOx concentration produced at equilibrium was 16.02 x 10(16) molecules/J (0.66 x 10(16) NO molecules/J and 15.36 x 10(16) NO2 molecules/J). Under the condition of the source gases consisting of NO and NO2 of 970 ppm in the N-2 and O-2 mixture with a ratio of 79/21, the concentrations of NOx generated were 5,571 and 5,320 ppm. (C) 2010 The Japan Society of Applied Physics
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页数:8
相关论文
共 31 条
[1]  
CHAMEIDES WL, 1977, J ATMOS SCI, V34, P143, DOI 10.1175/1520-0469(1977)034<0143:NPIL>2.0.CO
[2]  
2
[3]   Production of nitrogen oxides by a large spark generator [J].
Cook, DR ;
Liaw, YP ;
Sisterson, DL ;
Miller, NL .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2000, 105 (D6) :7103-7110
[4]   Efficiencies for production of NOx and O3 by streamer discharges in air at atmospheric pressure [J].
Cooray, V ;
Rahman, M .
JOURNAL OF ELECTROSTATICS, 2005, 63 (6-10) :977-983
[5]  
Fridman A., 2008, PLASMA CHEM
[6]  
Fridman A., 2004, Plasma Physics and Engineering
[7]   Blood coagulation and living tissue sterilization by floating-electrode dielectric barrier discharge in air [J].
Fridman, Gregory ;
Peddinghaus, Marie ;
Ayan, Halim ;
Fridman, Alexander ;
Balasubramanian, Manjula ;
Gutsol, Alexander ;
Brooks, Ari ;
Friedman, Gary .
PLASMA CHEMISTRY AND PLASMA PROCESSING, 2006, 26 (04) :425-442
[8]   Performance of a spark ignition engine fuelled with reformate gas produced on-board vehicle [J].
Galloni, Enzo ;
Minutillo, Mariagiovanna .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2007, 32 (13) :2532-2538
[9]   OZONE AND OXIDES OF NITROGEN-PRODUCTION DURING THUNDERSTORMS [J].
GRIFFING, GW .
JOURNAL OF GEOPHYSICAL RESEARCH-OCEANS AND ATMOSPHERES, 1977, 82 (06) :943-950
[10]   New continuous gas-phase synthesis of high purity carbon nanotubes by a thermal plasma jet [J].
Hahn, J ;
Han, JH ;
Yoo, JE ;
Jung, HY ;
Suh, JS .
CARBON, 2004, 42 (04) :877-883