Persistent memory for a Brownian walker in a random array of obstacles

被引:31
作者
Franosch, Thomas [1 ,2 ,3 ]
Hoefling, Felix [4 ]
Bauer, Teresa [2 ,3 ]
Frey, Erwin [2 ,3 ]
机构
[1] Univ Erlangen Nurnberg, Inst Theoret Phys, D-91058 Erlangen, Germany
[2] Univ Munich, Arnold Sommerfeld Ctr Theoret Phys, Fak Phys, D-80333 Munich, Germany
[3] Univ Munich, Fak Phys, Ctr NanoSci CeNS, D-80333 Munich, Germany
[4] Rudolf Peierls Ctr Theoret Phys, Oxford OX1 3NP, England
关键词
Brownian motion; Disordered solids; Computer simulation; VELOCITY AUTOCORRELATION FUNCTION; LORENTZ GAS; DIFFUSION-COEFFICIENT; TRANSPORT-PROPERTIES; DENSITY EXPANSION; KINETIC-THEORY; MOTION; SUSPENSIONS; MOTORS; BEHAVIOUR;
D O I
10.1016/j.chemphys.2010.04.023
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We show that for particles performing Brownian motion in a frozen array of scatterers long-time correlations emerge in the mean-square displacement. Defining the velocity autocorrelation function (VACF) via the second time-derivative of the mean-square displacement, power-law tails govern the long-time dynamics similar to the case of ballistic motion. The physical origin of the persistent memory is due to repeated encounters with the same obstacle which occurs naturally in Brownian dynamics without involving other scattering centers. This observation suggests that in this case the VACF exhibits these anomalies already at first order in the scattering density. Here we provide an analytic solution for the dynamics of a tracer for a dilute planar Lorentz gas and compare our results to computer simulations. Our result support the idea that quenched disorder provides a generic mechanism for persistent correlations irrespective of the microdynamics of the tracer particle. Crown Copyright (C) 2010 Published by Elsevier B.V. All rights reserved.
引用
收藏
页码:540 / 547
页数:8
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