S-matrix theory of high harmonic generation and ionization of coherently ro-vibrating linear molecules by intense ultrashort laser pulses

被引：5
作者：
Faisal, F. H. M. [1 ]
机构：
[1] Univ Bielefeld, Fak Phys, D-33501 Bielefeld, Germany
来源：
THEORETICAL CHEMISTRY ACCOUNTS | 2010年 / 127卷 / 03期
关键词：
S-Matrix theory; High harmonic generation; Ionization; Ro-vibration; Intense; Ultrashort; Laser pulses; Pump-prove signal; Time-delay; Clock-motion; EXCITATION; DYNAMICS; FIELDS;
D O I：
10.1007/s00214-009-0712-z
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
A theory of high harmonic generation and ionization of coherently rotating and vibrating linear molecules by a delayed pair of intense ultrashort laser pulses is presented. It correlates the nuclear motions in real time with the modulation of the harmonic emission and ionization signals as a function of the time-delay between the exciting and the probing pulses. An illustrative analytical example of the excitation and detection of the clock-motion associated with the "0-1" vibrational oscillation of a diatomic molecule is also given.
引用
收藏
页码：175 / 182
页数：8
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