Three-dimensional spin fluctuations in Na0.75CoO2 -: art. no. 157206

被引:96
作者
Helme, LM [1 ]
Boothroyd, AT
Coldea, R
Prabhakaran, D
Tennant, DA
Hiess, A
Kulda, J
机构
[1] Univ Oxford, Dept Phys, Oxford OX1 3PU, England
[2] Univ St Andrews, Sch Phys & Astron, St Andrews KY16 9SS, Fife, Scotland
[3] Inst Max Von Laue Paul Langevin, F-38042 Grenoble, France
基金
英国工程与自然科学研究理事会;
关键词
D O I
10.1103/PhysRevLett.94.157206
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We report polarized- and unpolarized-neutron scattering measurements of magnetic excitations in single-crystal Na0.75CoO2. The data confirm ferromagnetic correlations within the cobalt layers and reveal antiferromagnetic correlations perpendicular to the layers, consistent with an A-type antiferromagnetic ordering. The magnetic modes propagating perpendicular to the layers are sharp, and reach a maximum energy of similar to 12 meV. From a minimal spin-wave model, containing only nearest-neighbor Heisenberg exchange interactions, we estimate the interlayer and intralayer exchange constants to be 12.2 +/- 0.5 meV and -6 +/- 2 meV, respectively. We conclude that the magnetic fluctuations in Na0.75CoO2 are highly three dimensional.
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页数:4
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