Carbon-Based Metal-Free Catalysts for Electrocatalysis beyond the ORR

被引:636
作者
Hu, Chuangang [1 ]
Dai, Liming [1 ]
机构
[1] Case Western Reserve Univ, Ctr Adv Sci & Engn Carbon Case4 Carbon, Dept Macromol Sci & Engn, 10900 Euclid Ave, Cleveland, OH 44106 USA
关键词
carbon nanomaterials; hydrogen evolution; metal-free catalysts; oxygen evolution; oxygen reduction; NITROGEN-DOPED CARBON; HYDROGEN-EVOLUTION REACTION; OXYGEN REDUCTION REACTION; ONE-STEP SYNTHESIS; IN-SITU FORMATION; GRAPHENE-BASED MATERIALS; HIGHLY-ACTIVE CATALYSTS; COBALT OXIDE; BIFUNCTIONAL ELECTROCATALYST; EFFICIENT ELECTROCATALYST;
D O I
10.1002/anie.201509982
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Besides their use in fuel cells for energy conversion through the oxygen reduction reaction (ORR), carbon-based metal-free catalysts have also been demonstrated to be promising alternatives to noble-metal/metal oxide catalysts for the oxygen evolution reaction (OER) in metal-air batteries for energy storage and for the splitting of water to produce hydrogen fuels through the hydrogen evolution reaction (HER). This Review focuses on recent progress in the development of carbon-based metal-free catalysts for the OER and HER, along with challenges and perspectives in the emerging field of metal-free electrocatalysis.
引用
收藏
页码:11736 / 11758
页数:23
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