Narrowband Perovskite Photodetector-Based Image Array for Potential Application in Artificial Vision

被引:224
作者
Xue, Jie [1 ]
Zhu, Zhengfeng [1 ]
Xu, Xiaobao [1 ]
Gu, Yu [1 ]
Wang, Shalong [1 ]
Xu, Leimeng [1 ]
Zou, Yousheng [1 ]
Song, Jizhong [1 ]
Zeng, Haibo [1 ]
Chen, Qian [2 ]
机构
[1] Nanjing Univ Sci & Technol, MIIT Key Lab Adv Display Mat & Devices, Coll Mat Sci & Engn, Inst Optoelect & Nanomat, Nanjing 210094, Jiangsu, Peoples R China
[2] Nanjing Univ Sci & Technol, Jiangsu Key Lab Spectral Imaging & Intelligence S, Nanjing 210094, Jiangsu, Peoples R China
基金
中国博士后科学基金;
关键词
All-inorganic perovskite; freeze-drying; polycrystalline films; narrowband photodetector; image sensor array; LIGHT; FILTERLESS; DETECTOR; FAMILY; FILMS;
D O I
10.1021/acs.nanolett.8b03209
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Image sensor arrays are widely used in digital cameras, smartphones, and biorobots. However, most commercial image arrays rely on the dichroic prisms or a set of interference filters to distinguish characteristic color spectrum, which significantly increases the cost and fabrication processing complexity. In this work, an ultranarrow response photodetector with full-width at half-maximum being similar to 12 nm and specific detectivity over 10(11) Jones at 545 nm are successfully achieved in CsPbBr3 polycrystalline films using freeze-drying casting method to adjust the surface-charge recombination. To our best knowledge, this is the narrowest spectrum response for perovskite photodetectors in the visible light waveband. More importantly, a series of narrowband photodetectors are developed to enhance diverse selectivity for target signals covering from blue light to red light via bandgap tuning in CsPbX3 by tailoring the halide component. Finally, an integrated sensing array with CsPbX3 (X = Cl, Br, I) narrowband photodetectors acting as color recognition cones is constructed, which presents clear color and shape recognition paving the way for commercialization of perovskite photodetector in artificial vision.
引用
收藏
页码:7628 / 7634
页数:7
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