Upconversion enhancement by a dual-resonance all-dielectric metasurface

被引:32
作者
Gong, Chensheng [1 ]
Liu, Wen [1 ]
He, Nan [1 ]
Dong, Hongguang [1 ]
Jin, Yi [1 ]
He, Sailing [1 ,2 ]
机构
[1] Zhejiang Univ, State Key Lab Modern Opt Instrumentat, Ctr Opt & Electromagnet Res, East Bldg 5,Zijingang Campus, Hangzhou 310058, Zhejiang, Peoples R China
[2] Royal Inst Technol KTH, JORCEP, Sch Elect Engn, S-10044 Stockholm, Sweden
基金
中国国家自然科学基金;
关键词
PLASMON ENHANCEMENT; FIELD ENHANCEMENT; IN-VIVO; NANOPARTICLES; LUMINESCENCE; EMISSION; NANOCRYSTALS; FLUORESCENCE;
D O I
10.1039/c8nr08653b
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Upconversion nanoparticles (UCNPs) have drawn much attention in the past decade due to their superior physicochemical features and great potential in biomedical and biophotonic studies. However, their low luminescence efficiency often limits their applications. Here, we demonstrated a dual-resonance all-dielectric metasurface to enhance the signals emitted by upconversion nanoparticles (NaYF4:Yb/Tm). An averaged upconversion signal enhancement of around 400 times is detected experimentally. The electric and magnetic dipole resonances of the metasurface are designed to enhance the local excitation field and the quantum efficiency of the upconversion nanoparticles, respectively. Furthermore, the collection efficiency is enhanced due to the directional emission of the UCNPs on the metasurface. Our approach provides a powerful tool to extend the sensing application potential of upconversion nanoparticles.
引用
收藏
页码:1856 / 1862
页数:7
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