Effects of heat and water transport on the performance of polymer electrolyte membrane fuel cell under high current density operation

被引:58
|
作者
Tabuchi, Yuichiro [1 ]
Shiomi, Takeshi [1 ]
Aoki, Osamu [1 ]
Kubo, Norio [1 ]
Shinohara, Kazuhiko [1 ]
机构
[1] Nissan Motor Co Ltd, EV Syst Lab, Nissan Res Ctr, Kanagawa 2378523, Japan
关键词
PEMFC; Water management; Neutron radiography; Multiphase mixture model; PREDICTION; SATURATION; MEDIA; SETUP;
D O I
10.1016/j.electacta.2010.08.070
中图分类号
O646 [电化学、电解、磁化学];
学科分类号
081704 ;
摘要
Key challenges to the acceptance of polymer electrolyte membrane fuel cells (PEMFCs) for automobiles are the cost reduction and improvement in its power density for compactness. In order to get the solution, the further improvement in a fuel cell performance is required. In particular, under higher current density operation, water and heat transport in PEMFCs has considerable effects on the cell performance. In this study, the impact of heat and water transport on the cell performance under high current density was investigated by experimental evaluation of liquid water distribution and numerical validation. Liquid water distribution in MEA between rib and channel area is evaluated by neutron radiography. In order to neglect the effect of liquid water in gas channels and reactant species concentration distribution in the flow direction, the differential cell was used in this study. Experimental results suggested that liquid water under the channel was dramatically changed with rib/channel width. From the numerical study, it is found that the change of liquid water distribution was significantly affected by temperature distribution in MEA between rib and channel area. In addition, not only heat transport but also water transport through the membrane also significantly affected the cell performance under high current density operation. (C) 2010 Elsevier Ltd. All rights reserved.
引用
收藏
页码:352 / 360
页数:9
相关论文
共 50 条
  • [21] Optimization of graded catalyst layer to enhance uniformity of current density and performance of high temperature-polymer electrolyte membrane fuel cell
    Babu, Venkatesh K.
    Varghese, Geethu
    Joseph, Thadathil Varghese
    Chippar, Purushothama
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2022, 47 (06) : 4018 - 4032
  • [22] On the modeling of water transport in polymer electrolyte membrane fuel cells
    Wu, Hao
    Li, Xianguo
    Berg, Peter
    ELECTROCHIMICA ACTA, 2009, 54 (27) : 6913 - 6927
  • [23] Effects of membrane electrode assembly preparation on the polymer electrolyte membrane fuel cell performance
    Frey, T
    Linardi, M
    ELECTROCHIMICA ACTA, 2004, 50 (01) : 99 - 105
  • [24] Effects of Cracks on the Mass Transfer of Polymer Electrolyte Membrane Fuel Cell with High Performance Membrane Electrode Assembly
    Jinrong Shi
    Zhigang Zhan
    Di Zhang
    Yuan Yu
    Xiaoxiang Yang
    Luyan He
    Mu Pan
    Journal of Wuhan University of Technology-Mater. Sci. Ed., 2021, 36 : 318 - 330
  • [25] Effects of Cracks on the Mass Transfer of Polymer Electrolyte Membrane Fuel Cell with High Performance Membrane Electrode Assembly
    施金蓉
    詹志刚
    ZHANG Di
    YU Yuan
    YANG Xiaoxiang
    HE Luyan
    PAN Mu
    JournalofWuhanUniversityofTechnology(MaterialsScience), 2021, 36 (03) : 318 - 330
  • [26] Effects of Cracks on the Mass Transfer of Polymer Electrolyte Membrane Fuel Cell with High Performance Membrane Electrode Assembly
    Shi Jinrong
    Zhan Zhigang
    Zhang Di
    Yu Yuan
    Yang Xiaoxiang
    He Luyan
    Pan Mu
    JOURNAL OF WUHAN UNIVERSITY OF TECHNOLOGY-MATERIALS SCIENCE EDITION, 2021, 36 (03): : 318 - 330
  • [27] Performance of polymer electrolyte membrane fuel cell stack
    Chu, D
    Jiang, RZ
    PROCEEDINGS OF THE SECOND INTERNATIONAL SYMPOSIUM ON PROTON CONDUCTING MEMBRANE FUEL CELL II, 1999, 98 (27): : 470 - +
  • [28] Performance of polymer electrolyte membrane for polymer electrolyte fuel cell membrane made with supramolecular structure
    Hendrana, S.
    Indayaningsih, N.
    Sudirman
    INTERNATIONAL SYMPOSIUM ON FRONTIER OF APPLIED PHYSICS, 2018, 2019, 1191
  • [29] High Resolution Neutron Imaging of Water in the Polymer Electrolyte Fuel Cell Membrane
    Mukherjee, P. P.
    Mukundan, R.
    Spendelow, J. S.
    Davey, J. R.
    Borup, R. L.
    Hussey, D. S.
    Jacobson, D. L.
    Arif, M.
    PROTON EXCHANGE MEMBRANE FUEL CELLS 9, 2009, 25 (01): : 505 - 512
  • [30] Magnetic field effects on the performance of polymer electrolyte membrane fuel cell systems
    Leddy, J
    Gellett, WL
    Dunwoody, DC
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2004, 227 : U79 - U79