High-Gain and Low-Driving-Voltage Photodetectors Based on Organolead Triiodide Perovskites

被引:808
作者
Dong, Rui [1 ]
Fang, Yanjun [1 ]
Chae, Jungseok [2 ,3 ]
Dai, Jun [4 ]
Xiao, Zhengguo [1 ]
Dong, Qingfeng [1 ]
Yuan, Yongbo [1 ]
Centrone, Andrea [2 ]
Zeng, Xiao Cheng [1 ,4 ]
Huang, Jinsong [1 ]
机构
[1] Univ Nebraska, Dept Mech & Mat Engn, Lincoln, NE 68588 USA
[2] NIST, Ctr Nanoscale Sci & Technol, Gaithersburg, MD 20899 USA
[3] Univ Maryland, Maryland Nanoctr, College Pk, MD 20742 USA
[4] Univ Nebraska, Dept Chem, Lincoln, NE 68588 USA
基金
美国国家科学基金会;
关键词
SOLAR-CELLS; TEMPERATURE; NANOSCALE; POLYMER;
D O I
10.1002/adma.201405116
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Solution-processed organometal trihalide perovskite photodetectors show a high photoconductive gain of above 400 across the UV to NIR range at a very low bias of 1 V. The charge traps caused by large concentrations of Pb2+ cations at the top surface of the perovskite film are critical for achieving high gain in these devices via a trapped-hole-induced electron injection mechanism.
引用
收藏
页码:1912 / +
页数:8
相关论文
共 33 条
  • [1] Organic Light Detectors: Photodiodes and Phototransistors
    Baeg, Kang-Jun
    Binda, Maddalena
    Natali, Dario
    Caironi, Mario
    Noh, Yong-Young
    [J]. ADVANCED MATERIALS, 2013, 25 (31) : 4267 - 4295
  • [2] Synthesis and crystal chemistry of the hybrid perovskite (CH3NH3) PbI3 for solid-state sensitised solar cell applications
    Baikie, Tom
    Fang, Yanan
    Kadro, Jeannette M.
    Schreyer, Martin
    Wei, Fengxia
    Mhaisalkar, Subodh G.
    Graetzel, Michael
    White, Tim J.
    [J]. JOURNAL OF MATERIALS CHEMISTRY A, 2013, 1 (18) : 5628 - 5641
  • [3] Understanding the formation and evolution of interdiffusion grown organolead halide perovskite thin films by thermal annealing
    Bi, Cheng
    Shao, Yuchuan
    Yuan, Yongbo
    Xiao, Zhengguo
    Wang, Chenggong
    Gao, Yongli
    Huang, Jinsong
    [J]. JOURNAL OF MATERIALS CHEMISTRY A, 2014, 2 (43) : 18508 - 18514
  • [4] PROJECTOR AUGMENTED-WAVE METHOD
    BLOCHL, PE
    [J]. PHYSICAL REVIEW B, 1994, 50 (24): : 17953 - 17979
  • [5] Sequential deposition as a route to high-performance perovskite-sensitized solar cells
    Burschka, Julian
    Pellet, Norman
    Moon, Soo-Jin
    Humphry-Baker, Robin
    Gao, Peng
    Nazeeruddin, Mohammad K.
    Graetzel, Michael
    [J]. NATURE, 2013, 499 (7458) : 316 - +
  • [6] Nanoparticle-assisted high photoconductive gain in composites of polymer and fullerene
    Chen, Hsiang-Yu
    Lo, Michael K. F.
    Yang, Guanwen
    Monbouquette, Harold G.
    Yang, Yang
    [J]. NATURE NANOTECHNOLOGY, 2008, 3 (09) : 543 - 547
  • [7] Anode interfacial engineering approaches to enhancing anode/hole transport layer interfacial stability and charge injection efficiency in organic light-emitting diodes
    Cui, J
    Huang, QL
    Veinot, JCG
    Yan, H
    Wang, QW
    Hutchison, GR
    Richter, AG
    Evmenenko, G
    Dutta, P
    Marks, TJ
    [J]. LANGMUIR, 2002, 18 (25) : 9958 - 9970
  • [8] Local infrared microspectroscopy with subwavelength spatial resolution with an atomic force microscope tip used as a photothermal sensor
    Dazzi, A
    Prazeres, R
    Glotin, E
    Ortega, JM
    [J]. OPTICS LETTERS, 2005, 30 (18) : 2388 - 2390
  • [9] Van der Waals density functional for general geometries -: art. no. 246401
    Dion, M
    Rydberg, H
    Schröder, E
    Langreth, DC
    Lundqvist, BI
    [J]. PHYSICAL REVIEW LETTERS, 2004, 92 (24) : 246401 - 1
  • [10] An Ultraviolet-to-NIR Broad Spectral Nanocomposite Photodetector with Gain
    Dong, Rui
    Bi, Cheng
    Dong, Qingfeng
    Guo, Fawen
    Yuan, Yongbo
    Fang, Yanjun
    Xiao, Zhengguo
    Huang, Jinsong
    [J]. ADVANCED OPTICAL MATERIALS, 2014, 2 (06): : 549 - 554