A novel back-trajectory analysis of the origin of black carbon transported to the Himalayas and Tibetan Plateau during 1996-2010

被引:94
作者
Lu, Zifeng [1 ]
Streets, David G. [1 ]
Zhang, Qiang [3 ,4 ]
Wang, Siwen [2 ]
机构
[1] Argonne Natl Lab, Decis & Informat Sci Div, Argonne, IL 60439 USA
[2] Tsinghua Univ, Sch Environm, Beijing 100084, Peoples R China
[3] Tsinghua Univ, Minist Educ Key Lab Earth Syst Modeling, Beijing 100084, Peoples R China
[4] Tsinghua Univ, Ctr Earth Syst Sci, Beijing 100084, Peoples R China
关键词
AEROSOLS; EMISSIONS; CHINA; MODEL; DEPOSITION; GLACIERS; RECORD; INDIA; SNOW;
D O I
10.1029/2011GL049903
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
Black carbon (BC) deposited on snow and ice accelerates glacier melting and contributes to climate change of the Himalayas and Tibetan Plateau (HTP). Taking into account emissions, hydrophilic-to-hydrophobic conversion, and removal processes of BC, a novel back-trajectory approach is developed to study the origin of BC reaching the HTP. The results indicate that BC received by the HTP increased by 41% from 1996 to 2010, implying that the BC problem is accelerating in the HTP region. South Asia and East Asia are the main source regions, accounting for 67% and 17% of BC transported to the HTP on an annual basis, followed by Former USSR (similar to 8%), Middle East (similar to 4%), Europe (similar to 2%), and Northern Africa (similar to 1%). BC reaching the HTP is high in winter and low in summer, and the relative contributions of different source regions vary with seasons. We show the seasonal spatial distribution of BC sources directly on a 0.5 degrees x 0.5 degrees grid, which provides information to policymakers about the best target areas for mitigating the climate changes and other effects on the HTP. Citation: Lu, Z., D. G. Streets, Q. Zhang, and S. Wang (2012), A novel back-trajectory analysis of the origin of black carbon transported to the Himalayas and Tibetan Plateau during 1996-2010, Geophys. Res. Lett., 39, L01809, doi:10.1029/2011GL049903.
引用
收藏
页数:6
相关论文
共 22 条
[1]   Light absorption by pollution, dust, and biomass burning aerosols: a global model study and evaluation with AERONET measurements [J].
Chin, Mian ;
Diehl, T. ;
Dubovik, O. ;
Eck, T. F. ;
Holben, B. N. ;
Sinyuk, A. ;
Streets, D. G. .
ANNALES GEOPHYSICAE, 2009, 27 (09) :3439-3464
[2]   Construction of a 1° x 1° fossil fuel emission data set for carbonaceous aerosol and implementation and radiative impact in the ECHAM4 model [J].
Cooke, WF ;
Liousse, C ;
Cachier, H ;
Feichter, J .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1999, 104 (D18) :22137-22162
[3]  
Draxler RR, 1998, AUST METEOROL MAG, V47, P295
[4]   Springtime warming and reduced snow cover from carbonaceous particles [J].
Flanner, M. G. ;
Zender, C. S. ;
Hess, P. G. ;
Mahowald, N. M. ;
Painter, T. H. ;
Ramanathan, V. ;
Rasch, P. J. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2009, 9 (07) :2481-2497
[5]   CHARACTERISTICS OF THE LOW-LEVEL TEMPERATURE INVERSION ALONG THE ALASKAN ARCTIC COAST [J].
KAHL, JD .
INTERNATIONAL JOURNAL OF CLIMATOLOGY, 1990, 10 (05) :537-548
[6]   Origin and radiative forcing of black carbon transported to the Himalayas and Tibetan Plateau [J].
Kopacz, M. ;
Mauzerall, D. L. ;
Wang, J. ;
Leibensperger, E. M. ;
Henze, D. K. ;
Singh, K. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2011, 11 (06) :2837-2852
[7]   Historical (1850-2000) gridded anthropogenic and biomass burning emissions of reactive gases and aerosols: methodology and application [J].
Lamarque, J. -F. ;
Bond, T. C. ;
Eyring, V. ;
Granier, C. ;
Heil, A. ;
Klimont, Z. ;
Lee, D. ;
Liousse, C. ;
Mieville, A. ;
Owen, B. ;
Schultz, M. G. ;
Shindell, D. ;
Smith, S. J. ;
Stehfest, E. ;
Van Aardenne, J. ;
Cooper, O. R. ;
Kainuma, M. ;
Mahowald, N. ;
McConnell, J. R. ;
Naik, V. ;
Riahi, K. ;
van Vuuren, D. P. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2010, 10 (15) :7017-7039
[8]   Enhanced surface warming and accelerated snow melt in the Himalayas and Tibetan Plateau induced by absorbing aerosols [J].
Lau, William K. M. ;
Kim, Maeng-Ki ;
Kim, Kyu-Myong ;
Lee, Woo-Seop .
ENVIRONMENTAL RESEARCH LETTERS, 2010, 5 (02)
[9]   Constraints from 210Pb and 7Be on wet deposition and transport in a global three-dimensional chemical tracer model driven by assimilated meteorological fields [J].
Liu, HY ;
Jacob, DJ ;
Bey, I ;
Yantosca, RM .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2001, 106 (D11) :12109-12128
[10]   Sulfur dioxide and primary carbonaceous aerosol emissions in China and India, 1996-2010 [J].
Lu, Z. ;
Zhang, Q. ;
Streets, D. G. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2011, 11 (18) :9839-9864