Spontaneous striped pattern formation in thin chiral nematic liquid crystal layers

被引:15
作者
Biagio, R. L. [1 ]
De Souza, R. T. [2 ]
Evangelista, L. R. [1 ]
Ribeiro de Almeida, R. R. [2 ]
Zola, R. S. [1 ,2 ]
机构
[1] Univ Estadual Maringa, Dept Fis, Ave Colombo 5790, BR-87020900 Maringa, Parana, Brazil
[2] Univ Tecnol Fed Parana, Dept Fis, Rua Marcilio Dias 635, BR-86812460 Apucarana, PR, Brazil
基金
巴西圣保罗研究基金会;
关键词
Stripes pattern formation; Wetting transition; Monte Carlo simulation; COMPUTER-SIMULATION; LATTICE MODEL; ANCHORING ENERGY; PHASE; POTENTIALS; INTERFACE; LIGHT; CELL;
D O I
10.1016/j.molliq.2018.08.029
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Periodic modulations in chiral nematic liquid crystals (CLCs) are used in several optical and photonic devices. A remarkable way of fabricating and controlling such patterns is in a thin wetting layer that grows as temperature is decreased. Here, we study this stripe formation process experimentally and by means of Monte Carlo simulations. We report on samples of CLCs that present, after the wetting transition, a stripe/fringe formation occurring either through a nucleation process or homogeneously across the cell. These patterns depend on the ratio of the pitch to thickness of the layer, elastic anisotropy, and anchoring strength. Although such process is well documented for CLCs under applied field, we show here that similar textural transitions occur in thin layers mediated by the weak anchoring at the CLC-isotropic interface; it happens for values of pitch to thickness ratio much smaller than the ones reported in field driven situation. The Monte Carlo method takes action in simulating the experimentally observed textures by using a pairwise additive potential model for CLCs. A qualitative comparison with the experimental phenomena is possible to be made in which both the stripes formation and their behavior agree with the experiments. (C) 2018 Elsevier B.V. All rights reserved.
引用
收藏
页码:703 / 711
页数:9
相关论文
共 54 条
[1]   A laboratory model of Saturn's North Polar Hexagon [J].
Aguiar, Ana C. Barbosa ;
Read, Peter L. ;
Wordsworth, Robin D. ;
Salter, Tara ;
Yamazaki, Y. Hiro .
ICARUS, 2010, 206 (02) :755-763
[2]   Pattern Formation in Nature: Physical Constraints and Self-Organising Characteristics [J].
Ball, Philip .
ARCHITECTURAL DESIGN, 2012, 82 (02) :22-27
[3]   Structure of water; A Monte Carlo calculation [J].
Barker, J. A. ;
Watts, R. O. .
CHEMICAL PHYSICS LETTERS, 1969, 3 (03) :144-145
[4]   COMPUTER-SIMULATIONS OF NEMATIC DROPLETS WITH BIPOLAR BOUNDARY-CONDITIONS [J].
BERGGREN, E ;
ZANNONI, C ;
CHICCOLI, C ;
PASINI, P ;
SEMERIA, F .
PHYSICAL REVIEW E, 1994, 50 (04) :2929-2939
[5]   Structure of the cholesteric-isotropic interface [J].
Bernardino, Nelson Rei ;
Figueirinhas Pereira, Maria Carolina ;
Silvestre, Nuno Miguel ;
Telo da Gama, Margarida Maria .
SOFT MATTER, 2014, 10 (47) :9399-9402
[6]   Role of the surface anchoring energy on the spontaneous modulated pattern formation of hybrid aligned cholesteric liquid crystals [J].
Biagio, R. L. ;
Teixeira de Souza, R. ;
Evangelista, L. R. ;
Zola, R. S. .
MOLECULAR CRYSTALS AND LIQUID CRYSTALS, 2017, 657 (01) :107-115
[7]   Computer simulation of a nematic hybrid cell: The effects of elastic anisotropy [J].
Chiccoli, C. ;
Evangelista, L. R. ;
Omori, E. K. ;
Pasini, P. ;
Teixeira-Souza, R. T. ;
Zannoni, C. .
MOLECULAR CRYSTALS AND LIQUID CRYSTALS, 2017, 649 (01) :86-93
[8]   COSMOLOGY IN THE LABORATORY - DEFECT DYNAMICS IN LIQUID-CRYSTALS [J].
CHUANG, I ;
DURRER, R ;
TUROK, N ;
YURKE, B .
SCIENCE, 1991, 251 (4999) :1336-1342
[9]   Alignment layers with variable anchoring strengths from Polyvinyl Alcohol [J].
Cui, Yue ;
Zola, Rafael S. ;
Yang, Young-Cheol ;
Yang, Deng-Ke .
JOURNAL OF APPLIED PHYSICS, 2012, 111 (06)
[10]   Surface induced twist in nematic and chiral nematic liquid crystals: stick-slip-like and constrained motion [J].
de Souza, R. F. ;
Lenzi, E. K. ;
de Souza, R. T. ;
Evangelista, L. R. ;
Li, Q. ;
Zola, R. S. .
SOFT MATTER, 2018, 14 (11) :2084-2093