Two isomeric and distinguishable H2S fluorescence probes for monitoring spoilage of eggs and visualizing exogenous and endogenous H2S in living cells

被引：0

作者：

He, Yuqian ^{[1
]}

Zhao, Bing ^{[1
]}

Kan, Wei ^{[1
]}

Ding, Limin ^{[2
]}

Yu, Zhaochuan ^{[1
]}

Wang, Mingyue ^{[1
]}

Song, Bo ^{[1
]}

Wang, Liyan ^{[1
]}

机构：

[1] Qiqihar Univ, Chem & Chem Engn Inst, Qiqihar 161006, Peoples R China

[2] First Hosp Qiqihar City, Cadre Ward, Qiqihar 161005, Peoples R China

来源：

ANALYST | 2020年 / 145卷 / 01期

基金：

中国国家自然科学基金;

关键词：

HYDROGEN-SULFIDE; SULFUR-COMPOUNDS; IN-VIVO; GAS; MITOCHONDRIA; METABOLISM; GENERATION; THIOLYSIS; SENSORS; FE3+;

D O I：

10.1039/c9an01629e

中图分类号：

O65 [分析化学];

学科分类号：

070302 ; 081704 ;

摘要：

Accurate fabrication of fluorescence probes to efficiently monitor and detect H2S levels in the fields of foodstuffs and physiology is crucial. Herein, we report two isomeric phenanthro[9,10-d]imidazole benzene sulfonamide-derived fluorescence probes (PI-2-SA and PI-4-SA), both of which display remarkable responses toward H2S over other analytes. The spectral characteristics of the two probes were investigated and are discussed in detail. By comparison, PI-2-SA was specific, sensitive (the limit of detection was ca. 12.3 nM), rapid (within <= 3 min) and dynamic (the rate constant was 0.02 s(-1)). Significantly, PI-2-SA was proved to be effective in monitoring the shelf-time progress of egg samples in real time as well as in the imaging of exogenous and endogenous H2S in HeLa cells.

引用

页码：213 / 222

页数：10

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