High-pressure and temperature dependence of dielectric relaxation in supercooled di-isobutyl phthalate

被引:49
作者
Paluch, M
Ziolo, J
Rzoska, SJ
Habdas, P
机构
[1] Institute of Physics, Silesian University, Katowice, 40-007
来源
PHYSICAL REVIEW E | 1996年 / 54卷 / 04期
关键词
D O I
10.1103/PhysRevE.54.4008
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
Results are presented for isothermal, high-pressure (up to p=300 MPa), and temperature (under atmospheric pressure) measurements of complex dielectric permittivity in supercooled di-isobutyl phthalate. The relaxation times determined from the temperature study obey the temperature Vogel-Fulcher-Tammann (VFT) law. The pressure dependence of relaxation times describes the relation tau=tau(0)exp[B/(p-P-o)] This equation gives the same ideal glass transition pressure po as the generalized VFT formula proposed by Leyser et al. [Phys. Rev. E 51, 5899 (1995)]. For isobaric and isothermal absorption curves, the scaling behavior has been also tested.
引用
收藏
页码:4008 / 4010
页数:3
相关论文
共 15 条
[2]  
Anisimov M.A., 1992, CRITICAL PHENOMENA L
[3]   LIQUID-GLASS TRANSITION, A FREE-VOLUME APPROACH [J].
COHEN, MH ;
GREST, GS .
PHYSICAL REVIEW B, 1979, 20 (03) :1077-1098
[4]   PRESSURE AND TEMPERATURE-DEPENDENT VISCOSITY OF 2 GLASS-FORMING LIQUIDS - GLYCEROL AND DIBUTYL PHTHALATE [J].
COOK, RL ;
KING, HE ;
HERBST, CA ;
HERSCHBACH, DR .
JOURNAL OF CHEMICAL PHYSICS, 1994, 100 (07) :5178-5189
[5]   SCALING IN THE RELAXATION OF SUPERCOOLED LIQUIDS [J].
DIXON, PK ;
WU, L ;
NAGEL, SR ;
WILLIAMS, BD ;
CARINI, JP .
PHYSICAL REVIEW LETTERS, 1990, 65 (09) :1108-1111
[6]   Analysis of recent measurements of the viscosity of glasses [J].
Fulcher, GS .
JOURNAL OF THE AMERICAN CERAMIC SOCIETY, 1925, 8 (06) :339-355
[7]   Analysis of recent measurements of the viscosity of glasses. II [J].
Fulcher, GS .
JOURNAL OF THE AMERICAN CERAMIC SOCIETY, 1925, 8 (12) :789-794
[8]   PRESSURE-DEPENDENT AND TEMPERATURE-DEPENDENT HOMODYNE PHOTON-CORRELATION STUDIES OF LIQUID ORTHO-TERPHENYL IN THE SUPERCOOLED STATE [J].
FYTAS, G ;
DORFMULLER, T ;
WANG, CH .
JOURNAL OF PHYSICAL CHEMISTRY, 1983, 87 (24) :5041-5045
[9]  
HAVRILIAK S, 1966, J POLYMER SCI C, V14, P99, DOI DOI 10.1002/POLC.5070140111
[10]   HIGH-PRESSURE SPECIFIC-HEAT SPECTROSCOPY AT THE GLASS-TRANSITION IN O-TERPHENYL [J].
LEYSER, H ;
SCHULTE, A ;
DOSTER, W ;
PETRY, W .
PHYSICAL REVIEW E, 1995, 51 (06) :5899-5904