Negative differential conductance and hot phonons in suspended nanotube molecular wires

被引:386
作者
Pop, E [1 ]
Mann, D
Cao, J
Wang, Q
Goodson, KE
Dai, HJ
机构
[1] Stanford Univ, Dept Chem, Stanford, CA 94305 USA
[2] Stanford Univ, Adv Mat Lab, Stanford, CA 94305 USA
[3] Stanford Univ, Dept Mech Engn & Thermal Sci, Stanford, CA 94305 USA
关键词
D O I
10.1103/PhysRevLett.95.155505
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Freely suspended metallic single-walled carbon nanotubes (SWNTs) exhibit reduced current carrying ability compared to those lying on substrates, and striking negative differential conductance at low electric fields. Theoretical analysis reveals significant self-heating effects including electron scattering by hot nonequilibrium optical phonons. Electron transport characteristics under strong self-heating are exploited for the first time to probe the thermal conductivity of individual SWNTs (similar to 3600 W m(-1) K-1 at T=300 K) up to similar to 700 K, and reveal a 1/T dependence expected for umklapp phonon scattering at high temperatures.
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页数:4
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