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Wet Deposition of Fission-Product Isotopes to North America from the Fukushima Dai-ichi Incident, March 2011
被引:24
|作者:
Wetherbee, Gregory A.
[1
]
Gay, David A.
[2
]
Debey, Timothy M.
[3
]
Lehmann, Christopher M. B.
[2
]
Nilles, Mark A.
[4
]
机构:
[1] US Geol Survey, Branch Qual Syst, Denver Fed Ctr, Lakewood, CO 80225 USA
[2] Univ Illinois, Illinois State Water Survey, Natl Atmospher Deposit Program, Champaign, IL 61820 USA
[3] US Geol Survey, Natl Reactor Facil, Denver Fed Ctr, Lakewood, CO 80225 USA
[4] US Geol Survey, Off Water Qual, Denver Fed Ctr, Lakewood, CO 80225 USA
基金:
美国食品与农业研究所;
关键词:
NUCLEAR-POWER-PLANT;
CHERNOBYL ACCIDENT;
DRY DEPOSITION;
FALLOUT;
CS-137;
I-131;
RECONSTRUCTION;
TRANSPORT;
CESIUM;
SOILS;
D O I:
10.1021/es203217u
中图分类号:
X [环境科学、安全科学];
学科分类号:
08 ;
0830 ;
摘要:
Using the infrastructure of the National Atmospheric Deposition Program (NADP), numerous measurements of radionuclide wet deposition over North America were made for 167 NADP sites before and after the Fukushima Dai-ichi Nuclear Power Station incident of March 12, 2011. For the period from March 8 through April 5, 2011, wet-only precipitation samples were collected by NADP and analyzed for fission-product isotopes within whole-water and filterable solid samples by the United States Geological Survey using gamma spectrometry. Variable amounts of I-131, Cs-134, or Cs-137 were measured at approximately 21% of sampled NADP sites distributed widely across the contiguous United States and Alaska. Calculated 1- to 2-week individual radionuclide deposition fluxes ranged from 0.47 to 5100 Becquerels per square meter during the sampling period. Wet deposition activity was small compared to measured activity already present in U.S. soil. NADP networks responded to this complex disaster, and provided scientifically valid measurements that are comparable and complementary to other networks in North America and Europe.
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页码:2574 / 2582
页数:9
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