Atomic-scale imaging in real and energy space developed in ultrafast electron microscopy

被引:75
作者
Park, Hyun Soon [1 ]
Baskin, J. Spencer [1 ]
Kwon, Oh-Hoon [1 ]
Zewail, Ahmed H. [1 ]
机构
[1] CALTECH, Phys Biol Ctr Ultrfast Sci & Technol, Arthur Amos Noyes Lab Chem Phys, Pasadena, CA 91125 USA
关键词
D O I
10.1021/nl071369q
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
In this contribution, we report the development of ultrafast electron microscopy (UEM) with atomic-scale real-, energy-, and Fourier-space resolutions. This second-generation UEM provides images, diffraction patterns, and electron energy spectra, and here we demonstrate its potential with applications for nanostructured materials and organometallic crystals. We clearly resolve the separation between atoms in the direct images and the Bragg spots/Debye-Scherrer rings in diffraction and obtain the electronic structure and elemental energies in the electron energy loss spectra (EELS) and energy filtered transmission electron microscopy (EFTEM).
引用
收藏
页码:2545 / 2551
页数:7
相关论文
共 22 条
[1]  
[Anonymous], 1998, HIGH RESOLUTION ELEC
[2]   Breaking resolution limits in ultrafast electron diffraction and microscopy [J].
Baum, Peter ;
Zewail, Ahmed H. .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2006, 103 (44) :16105-16110
[3]  
BRYDSON R, 2001, ELECTRON ENERGY LOSS
[4]  
GEDIK N, 2007, SCIENCE, V7, P2552
[5]   Four-dimensional ultrafast electron microscopy of phase transitions [J].
Grinolds, Michael S. ;
Lobastov, Vladimir A. ;
Weissenrieder, Jonas ;
Zewail, Ahmed H. .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2006, 103 (49) :18427-18431
[6]   Direct imaging of transient molecular structures with ultrafast diffraction [J].
Ihee, H ;
Lobastov, VA ;
Gomez, UM ;
Goodson, BM ;
Srinivasan, R ;
Ruan, CY ;
Zewail, AH .
SCIENCE, 2001, 291 (5503) :458-462
[7]   Four-dimensional ultrafast electron microscopy [J].
Lobastov, VA ;
Srinivasan, R ;
Zewail, AH .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2005, 102 (20) :7069-7073
[8]   Ultrafast electron microscopy (UEM): Four-dimensional imaging and diffraction of nanostructures during phase transitions [J].
Lobastov, Vladimir A. ;
Weissenrieder, Jonas ;
Tang, Jau ;
Zewail, Ahmed H. .
NANO LETTERS, 2007, 7 (09) :2552-2558
[9]  
MURATA Y, 1977, ACTA CRYSTALLOGR A, V33, P198, DOI 10.1107/S0567739477000400
[10]   MOLECULAR IMAGING OF DISLOCATIONS IN 16 CHLOROCOPPER PHTHALOCYANINE [J].
MURATA, Y ;
BAIRD, T ;
FRYER, JR .
NATURE, 1976, 262 (5570) :721-722