Nitrogen-doped carbon nanoparticles derived from acrylonitrile plasma for electrochemical oxygen reduction

被引：76

作者：

Panomsuwan, Gasidit ^{[1
]}

Saito, Nagahiro ^{[2
,3
,4
]}

Ishizaki, Takahiro ^{[1
,4
]}

机构：

[1] Shibaura Inst Technol, Fac Engn, Dept Mat Sci & Engn, Tokyo 1358548, Japan

[2] Nagoya Univ, Grad Sch Engn, Dept Mat Phys & Energy Engn, Nagoya, Aichi 4648603, Japan

[3] Nagoya Univ, Green Mobil Collaborat Res Ctr, Nagoya, Aichi 4648603, Japan

[4] Japan Sci & Technol Agcy JST, CREST, Saitama 333001, Japan

来源：

PHYSICAL CHEMISTRY CHEMICAL PHYSICS | 2015年 / 17卷 / 09期

关键词：

HIGH ELECTROCATALYTIC ACTIVITY; METAL-FREE ELECTROCATALYSTS; OPTICAL-EMISSION; GRAPHENE; CATALYSTS; MECHANISMS; EVOLUTION; ARRAYS; OXIDE;

D O I：

10.1039/c4cp05995f

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Nitrogen-doped carbon nanoparticles were synthesized via a solution plasma process, with acrylonitrile as a single-source precursor, followed by a post-thermal annealing process. The nitrogen-bonding states can be tuned by varying the annealing temperature. The best electrocatalytic activity for oxygen reduction reaction (ORR) in terms of both onset potential and limiting current density can be achieved for the catalyst annealed at an optimal temperature of 800 degrees C because of the high content of graphitic-N catalytic sites and a large specific surface area.

引用

页码：6227 / 6232

页数：6

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