Polycyclic aromatic hydrocarbons in urban soils of Beijing: Status, sources, distribution and potential risk

被引:429
作者
Peng, Chi [1 ]
Chen, Weiping [1 ]
Liao, Xiaolan [2 ]
Wang, Meie [1 ]
Ouyang, Zhiyun [1 ]
Jiao, Wentao [1 ]
Bai, Yang [1 ]
机构
[1] Chinese Acad Sci, Ecoenvironm Sci Res Ctr, State Key Lab Urban & Reg Ecol, Beijing 100085, Peoples R China
[2] Hunan Agr Univ, Coll Biosafety Sci & Technol, Changsha 410128, Hunan, Peoples R China
基金
中国国家自然科学基金;
关键词
PAHs; Principal component analysis; Kriging; Incremental lifetime cancer risks; Health risk assessment; Urban soil; AGRICULTURAL SOILS; POLLUTION SOURCES; CHINA; PAHS; RIVER; CONTAMINATION; TIANJIN; REGION; CARBON; CITY;
D O I
10.1016/j.envpol.2010.11.003
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
We studied the source, concentration, spatial distribution and health risk of 16 polycyclic aromatic hydrocarbons (PAHs) in urban soils of Beijing. The total mass concentration of 16 PAHs ranged from 93 to 13 141 mu g kg(-1) with a mean of 1228 mu g kg(-1). The contour map of soil PAH concentrations showed that the industrial zone, the historical Hutong district and the university district of Beijing have significantly higher concentrations than those in remainder of the city. The results of sources identification suggested that the primary sources of PAHs were vehicle exhaust and coal combustion and the secondary source was the atmospheric deposition of long-range transported PAHs. The incremental lifetime cancer risks (ILCRs) of exposing to PAHs in the urban soils of Beijing for adult were 1.77 x 10(-6) and 2.48 x 10(-5), respectively under normal and extreme conditions. For child, they were 8.87 x 10(-7) and 6.72 x 10(-6), respectively under normal and extreme conditions. Crown Copyright (C) 2010 Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:802 / 808
页数:7
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