A model on an entrained bed-bubbling bed process for CO2 capture from flue gas

被引:11
作者
Choi, Jeong-Hoo [1 ]
Yi, Chang-Keun [2 ]
Jo, Sung-Ho [2 ]
机构
[1] Konkuk Univ, Dept Chem Engn, Seoul 143701, South Korea
[2] Korea Inst Energy Res, Taejon 305343, South Korea
关键词
CO2; Capture; Model; Fluidized Bed; Entrained Bed; Sodium Carbonate; CARBON-DIOXIDE CAPTURE; SORBENT;
D O I
10.1007/s11814-010-0477-z
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A simplified model has been developed to investigate effects of important operating parameters on performance of an entrained-bed absorber and bubbling-bed regenerator system collecting CO2 from flue gas. The particle population balance was considered together with chemical reaction to determine the extent of conversion in both absorber and regenerator. The calculated CO2 capture efficiency agreed with the measured value reasonably well. Effects of absorber parameters - temperature, gas velocity, static bed height, moisture content of feed gas on CO2 capture efficiency - have been investigated in a laboratory scale process. The CO2 capture efficiency decreased as temperature or gas velocity increased. However, it increased with static bed height or moisture concentration. The CO2 capture efficiency was exponentially proportional to each parameter. Based on the absolute value of exponent of the parameter, the effect of gas velocity, static bed height, and moisture content was one-half, one-third, and one-fourth as strong as that of temperature, respectively.
引用
收藏
页码:1144 / 1147
页数:4
相关论文
共 17 条
[1]   Capturing CO2 from combustion flue gases with a carbonation calcination loop. Experimental results and process development [J].
Abanades, J. C. ;
Alonso, M. ;
Rodriguez, N. ;
Gonzalez, B. ;
Grasa, G. ;
Murillo, R. .
GREENHOUSE GAS CONTROL TECHNOLOGIES 9, 2009, 1 (01) :1147-1154
[2]   Modelling of a fluidized bed carbonator reactor to capture CO2 from a combustion flue gas [J].
Alonso, M. ;
Rodriguez, N. ;
Grasa, G. ;
Abanades, J. C. .
CHEMICAL ENGINEERING SCIENCE, 2009, 64 (05) :883-891
[3]  
Choi JH, 2005, KOREAN CHEM ENG RES, V43, P286
[4]   Correlation on the particle entrainment rate in gas fluidized beds [J].
Choi, JH ;
Chang, IY ;
Shun, DW ;
Yi, CK ;
Son, JE ;
Kim, SD .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1999, 38 (06) :2491-2496
[5]   Continuous CO2 Capture from Flue Gases Using a Dual Fluidized Bed Reactor with Calcium-Based Sorbent [J].
Fang, Fan ;
Li, Zhen-shan ;
Cai, Ning-sheng .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2009, 48 (24) :11140-11147
[6]  
Kunni D., 1991, FLUIDIZATION ENG, V2nd
[7]  
Lapple C.E., 1951, Chemical Engineering, V58, P144
[8]   Sodium-based dry regenerable sorbent for carbon dioxide capture from power plant flue gas [J].
Lee, Joong B. ;
Ryu, Chong K. ;
Baek, Jeom-In ;
Lee, Ji H. ;
Eom, Tae H. ;
Kim, Sung Hyun .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2008, 47 (13) :4465-4472
[9]  
Merrick D., 1974, AIChE Symp. Ser, V70, P366
[10]  
Park KW, 2009, KOREAN CHEM ENG RES, V47, P349