Momentum vector correlation maps for three-particle fragmentation of neutral triatomic hydrogen near its ionization threshold

被引:7
作者
Fechner, Peer [1 ]
Helm, Hanspeter [1 ]
机构
[1] Univ Freiburg, Dept Mol & Opt Phys, D-79104 Freiburg, Germany
来源
PHYSICAL REVIEW A | 2010年 / 82卷 / 05期
关键词
H-3; STATES; PHOTODISSOCIATION; PREDISSOCIATION; DISSOCIATION;
D O I
10.1103/PhysRevA.82.052523
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Three-particle dissociation of high-lying Rydberg states of H-3, in the immediate vicinity of the ionization threshold, is induced by an external electric field. We observe that the momentum vector correlation map of the center-of-mass motion of the fragments changes rapidly with electronic energy. Near-and above-threshold substantial contributions of fragment orientations which are characteristic of near-linear geometry appear, i.e., two atoms with opposing momenta, the third atom being nearly at rest. This finding is similar to observations by Strasser et al. [Phys. Rev. A 66, 032719 (2002)], who studied dissociative recombination of cold H-3(+) ions with slow electrons. We discuss the likely dissociation paths responsible for the observed correlation.
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页数:7
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