TiO2 nanoparticles and CQDs co-decorated mesoporous g-C3N4 and their photocatalytic properties for gaseous benzene degradation

被引:6
作者
Zhao, Chunxia [1 ]
Jia, Heng [1 ]
Jin, Wei [2 ]
Li, Feng [1 ]
Li, Hang [1 ]
Chen, Wen [1 ]
机构
[1] Wuhan Univ Technol, Sch Mat Sci & Engn, State Key Lab Adv Technol Mat Synth & Proc, Wuhan 430070, Hubei, Peoples R China
[2] Wuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Hubei, Peoples R China
基金
国家重点研发计划;
关键词
Mesoporous g-C3N4; TiO2; nanoparticles; carbon quantum dots; photocatalysis; gaseous benzene; IN-SITU SYNTHESIS; CARBON-DOTS; ULTRATHIN NANOSHEETS; HETEROJUNCTIONS; NANOCOMPOSITE; FABRICATION; NITRIDE;
D O I
10.1142/S1793604719500863
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Mesoporous g-C3N4 is prepared by a hard template method and is then decorated by carbon quantum dots (CQDs) and TiO2 nanoparticles through an impregnation route followed by a hydrothermal method. The synthesized hybrids possess higher specific surface area up to 131 cm(2)/g and show effective absorption of visible light range and improved instantaneous photocurrent response, which reveals the enhanced photo-generated carrier separation efficiency. The first-order kinetic reaction rate constant of photocatalytic degradation of gaseous benzene by TCPCN-2 is 5.5 times of the bulk g-C3N4. Its degradation rate is up to 96.08% with good photocatalytic stability. Thus, the TiO2 nanoparticles and CQDs co-decorated g-C3N4 hybrids are promising photocatalysts.
引用
收藏
页数:5
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