Reflection Electron Energy Loss Spectra beyond the optical limit

被引:2
作者
Calliari, Lucia [1 ,2 ]
Dapor, Maurizio [1 ,2 ]
Garberoglio, Giovanni [1 ,2 ]
Fanchenko, Sergey [3 ]
机构
[1] European Ctr Theoret Studies Nucl Phys & Related, I-38123 Trento, Italy
[2] Ist Nazl Fis Nucl, Trento Inst Fundamental Phys & Applicat, I-38123 Trento, Italy
[3] Kurchatov Inst, Natl Res Ctr, Moscow 123182, Russia
关键词
Inelastic scattering; Electron energy loss; Monte Carlo; Plasmon energy dispersion; Plasmon damping dispersion; BETHE SURFACE; SPECTROSCOPY; METALS; DEPENDENCE; SOLIDS; WATER; SI;
D O I
10.1016/j.nimb.2014.11.106
中图分类号
TH7 [仪器、仪表];
学科分类号
0804 ; 080401 ; 081102 ;
摘要
A position-dependent Inverse Inelastic Mean Free Path (IIMFP), calculated according to the Chen Kwei theory of inelastic scattering, is used to obtain Reflection Electron Energy Loss Spectra (REELS) by a Monte Carlo approach. The basic ingredient of the theory is the energy-loss and momentum-transfer dependent dielectric function, for which we use a plasmon-pole approximation to the Lindhard dielectric function. The dependence on the momentum transfer enters by assuming a proper dispersion relation for the energy loss. Experiments reveal however that, beside energy loss, also plasmon damping disperses with momentum transfer. By comparing measured and calculated REEL spectra, we explore the role of damping dispersion for a quasi-free-electron material like silicon. (C) 2014 Elsevier B.V. All rights reserved.
引用
收藏
页码:171 / 175
页数:5
相关论文
共 26 条
[1]  
[Anonymous], 2003, ELECT BEAM INTERACTI
[2]   OPTICAL-PROPERTIES OF SMALL METAL SPHERES - SURFACE EFFECTS [J].
APELL, P ;
PENN, DR .
PHYSICAL REVIEW LETTERS, 1983, 50 (17) :1316-1319
[3]  
Baltz R. V., 1997, NATO ASI SER, V356, P303
[4]   Reflection electron energy loss spectroscopy: role of the Bethe-Born factor [J].
Calliari, L. ;
Fanchenko, S. .
SURFACE AND INTERFACE ANALYSIS, 2012, 44 (08) :1104-1109
[5]   Momentum transfer dependence of reflection electron energy loss spectra: theory and experiment [J].
Calliari, Lucia ;
Dapor, Maurizio ;
Garberoglio, Giovanni ;
Fanchenko, Sergey .
SURFACE AND INTERFACE ANALYSIS, 2014, 46 (05) :340-349
[6]   Electron differential inverse mean free path for surface electron spectroscopy [J].
Chen, YF ;
Kwei, CM .
SURFACE SCIENCE, 1996, 364 (02) :131-140
[7]   Monte Carlo modeling of surface excitation in reflection electron energy loss spectroscopy spectrum for rough surfaces [J].
Da, B. ;
Mao, S. F. ;
Zhang, G. H. ;
Wang, X. P. ;
Ding, Z. J. .
JOURNAL OF APPLIED PHYSICS, 2012, 112 (03)
[8]  
Ding ZJ, 1996, SCANNING, V18, P92, DOI 10.1002/sca.1996.4950180204
[9]   DIRECT MEASUREMENT OF THE DIELECTRIC CONSTANTS OF SILICON AND GERMANIUM [J].
DUNLAP, WC ;
WATTERS, RL .
PHYSICAL REVIEW, 1953, 92 (06) :1396-1397
[10]  
Egerton R.F., 2011, ELECT ENERGY LOSS SP