High harmonic generation spectroscopy of hydrocarbons

被引:44
|
作者
Vozzi, C. [1 ]
Torres, R. [2 ]
Negro, M. [3 ]
Brugnera, L. [2 ]
Siegel, T. [2 ]
Altucci, C. [4 ,5 ]
Velotta, R. [4 ,5 ]
Frassetto, F. [6 ]
Poletto, L. [6 ]
Villoresi, P. [7 ]
De Silvestri, S. [3 ]
Stagira, S. [3 ]
Marangos, J. P. [2 ]
机构
[1] CNR IFN, I-20133 Milan, Italy
[2] Univ London Imperial Coll Sci Technol & Med, Blackett Lab, London SW7 2BW, England
[3] Politecn Milan, Dip Fis, I-20133 Milan, Italy
[4] Univ Naples Federico 2, I-80126 Naples, Italy
[5] CNISM, I-80126 Naples, Italy
[6] CNR IFN, I-35131 Padua, Italy
[7] Univ Padua, DEI, I-35131 Padua, Italy
基金
英国工程与自然科学研究理事会;
关键词
MOLECULES; DYNAMICS;
D O I
10.1063/1.3526752
中图分类号
O59 [应用物理学];
学科分类号
摘要
We have demonstrated the ability of few-cycle midinfrared intense laser pulses to produce extended harmonic spectra (>= 45 eV) suitable for high harmonic spectroscopy in aligned hydrocarbons with ionization potentials in the range 9.07-11.52 eV. Modulations in the spectra measured with different alignment angles show signatures of the molecular structure. These results pave the way for the extension of high harmonic spectroscopy to complex biomolecules. (C) 2010 American Institute of Physics. [doi:10.1063/1.3526752]
引用
收藏
页数:3
相关论文
共 50 条
  • [41] Opportunities for chiral discrimination using high harmonic generation in tailored laser fields
    Smirnova, Olga
    Mairesse, Yann
    Patchkovskii, Serguei
    JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2015, 48 (23)
  • [42] High-order harmonic generation from highly excited states in acetylene
    Mulholland, Peter
    Dundas, Daniel
    PHYSICAL REVIEW A, 2018, 97 (04)
  • [43] Extreme ultraviolet high-harmonic spectroscopy of solids
    Luu, T. T.
    Garg, M.
    Kruchinin, S. Yu.
    Moulet, A.
    Hassan, M. Th.
    Goulielmakis, E.
    NATURE, 2015, 521 (7553) : 498 - 502
  • [44] Anisotropic high-harmonic generation in bulk crystals
    You, Yong Sing
    Reis, David A.
    Ghimire, Shambhu
    NATURE PHYSICS, 2017, 13 (04) : 345 - 349
  • [45] High-order-harmonic generation of a doped semiconductor
    Huang, Tengfei
    Zhu, Xiaosong
    Li, Liang
    Liu, Xi
    Lan, Pengfei
    Lu, Peixiang
    PHYSICAL REVIEW A, 2017, 96 (04)
  • [46] High-Order Harmonic Generation and Attosecond Science
    Midorikawa, Katsumi
    JAPANESE JOURNAL OF APPLIED PHYSICS, 2011, 50 (09)
  • [47] Theoretical Analysis of High-Harmonic Generation in Solids
    Vampa, G.
    McDonald, C. R.
    Orlando, G.
    Klug, D. D.
    Corkum, P. B.
    Brabec, T.
    PHYSICAL REVIEW LETTERS, 2014, 113 (07)
  • [48] Effect of photoexcitation on high-harmonic generation in semiconductors
    de Keijzer, Brian
    van Essen, Pieter j.
    Kraus, Peter m.
    JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 2024, 41 (08) : 1754 - 1763
  • [49] Self-probing of molecules with high harmonic generation
    Haessler, S.
    Caillat, J.
    Salieres, P.
    JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2011, 44 (20)
  • [50] High-order harmonic generation by polyatomic molecules
    Odzak, S.
    Hasovic, E.
    Milosevic, D. B.
    25TH ANNUAL INTERNATIONAL LASER PHYSICS WORKSHOP (LPHYS'16), 2017, 826