High harmonic generation spectroscopy of hydrocarbons

被引:44
|
作者
Vozzi, C. [1 ]
Torres, R. [2 ]
Negro, M. [3 ]
Brugnera, L. [2 ]
Siegel, T. [2 ]
Altucci, C. [4 ,5 ]
Velotta, R. [4 ,5 ]
Frassetto, F. [6 ]
Poletto, L. [6 ]
Villoresi, P. [7 ]
De Silvestri, S. [3 ]
Stagira, S. [3 ]
Marangos, J. P. [2 ]
机构
[1] CNR IFN, I-20133 Milan, Italy
[2] Univ London Imperial Coll Sci Technol & Med, Blackett Lab, London SW7 2BW, England
[3] Politecn Milan, Dip Fis, I-20133 Milan, Italy
[4] Univ Naples Federico 2, I-80126 Naples, Italy
[5] CNISM, I-80126 Naples, Italy
[6] CNR IFN, I-35131 Padua, Italy
[7] Univ Padua, DEI, I-35131 Padua, Italy
基金
英国工程与自然科学研究理事会;
关键词
MOLECULES; DYNAMICS;
D O I
10.1063/1.3526752
中图分类号
O59 [应用物理学];
学科分类号
摘要
We have demonstrated the ability of few-cycle midinfrared intense laser pulses to produce extended harmonic spectra (>= 45 eV) suitable for high harmonic spectroscopy in aligned hydrocarbons with ionization potentials in the range 9.07-11.52 eV. Modulations in the spectra measured with different alignment angles show signatures of the molecular structure. These results pave the way for the extension of high harmonic spectroscopy to complex biomolecules. (C) 2010 American Institute of Physics. [doi:10.1063/1.3526752]
引用
收藏
页数:3
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