Optimization of radiolytic degradation of sulfadiazine by combining Fenton and gamma irradiation processes

被引：25

作者：

Barbaro Rivas-Ortiz, Iram ^{[1
]}

Cruz-Gonzalez, German ^{[1
]}

Lastre-Acosta, Arlen Mabel ^{[2
]}

Manduca-Artiles, Michel ^{[1
]}

Rapado-Paneque, Manuel ^{[3
]}

Chavez-Ardanza, Armando ^{[3
]}

Silva Costa Teixeira, Antonio Carlos ^{[2
]}

Jauregui-Haza, Ulises J. ^{[1
]}

机构：

[1] Univ Havana, Higher Inst Technol & Appl Sci, Havana, Cuba

[2] Univ Sao Paulo, Dept Chem Engn, Sao Paulo, Brazil

[3] Ctr Technol Applicat & Nucl Dev, Havana, Cuba

来源：

JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY | 2017年 / 314卷 / 03期

关键词：

Advanced oxidation processes; Gamma radiation; Fenton reaction; Hydrogen peroxide; Sulfadiazine; Process intensification; PERSONAL CARE PRODUCTS; AQUEOUS-SOLUTION; WASTE-WATER; PHARMACEUTICAL RESIDUES; ANTIBIOTIC-RESISTANCE; RISK-ASSESSMENT; RADIATION; DECOMPOSITION; REMOVAL; ENVIRONMENT;

D O I：

10.1007/s10967-017-5629-8

中图分类号：

O65 [分析化学];

学科分类号：

070302 ; 081704 ;

摘要：

Gamma radiation (GR) is a promising technique, among known advanced oxidation processes, degrading water contaminants. Nevertheless, few authors report the degradation of sulfonamides by GR, and limited information exists concerning the use of GR in the case of sulfadiazine (SDZ). The objectives of this work are (1) evaluating GR as an alternative method for treating wastewater contaminated with SDZ and examinating the intensification of GR with oxidants (H2O2 or Fenton reagent). GR was performed with a high-activity Co-60 source. The gamma radiation/Fenton process gave the best result, leading to total SDZ removal and high (74.13%) pollutant mineralization.

引用

页码：2597 / 2607

页数：11

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