Comparative study of gamma-ray shielding features and some properties of different heavy metal oxide-based tellurite-rich glass systems

被引:20
作者
Lakshminarayana, G. [1 ]
Kumar, Ashok [2 ]
Lira, A. [3 ]
Dahshan, A. [4 ,5 ]
Hegazy, H. H. [4 ,6 ]
Kityk, I., V [7 ]
Lee, Dong-Eun [8 ]
Yoon, Jonghun [9 ]
Park, Taejoon [10 ]
机构
[1] Kyungpook Natl Univ, Intelligent Construct Automat Ctr, 80 Daehak Ro, Daegu 41566, South Korea
[2] Univ Coll, Benra Dhuri, Punjab, India
[3] Univ Autonoma Estado Mexico, Fac Ciencias, Dept Fis, Toluca 50000, Mexico
[4] King Khalid Univ, Fac Sci, Dept Phys, POB 9004, Abha, Saudi Arabia
[5] Port Said Univ, Fac Sci, Dept Phys, Port Said, Egypt
[6] Al Azhar Univ, Fac Sci, Dept Phys, Assiut Branch, Assiut 71524, Egypt
[7] Czestochowa Tech Univ, Fac Elect Engn, Inst Optoelect & Measuring Syst, 17 Armii Krajowej Str, PL-42200 Czestochowa, Poland
[8] Kyungpook Natl Univ, Sch Architecture & Civil Engn, 80 Daehak Ro, Daegu 41566, South Korea
[9] Hanyang Univ, Dept Mech Engn, 80 Daehak Ro, Ansan 15588, Gyeonggi Do, South Korea
[10] Hanyang Univ, Dept Robot Engn, 55 Hanyangdaehak Ro, Ansan 15588, Gyeonggi Do, South Korea
基金
新加坡国家研究基金会;
关键词
Multicomponent tellurite glass; XRD; Raman spectroscopy; Mass attenuation coefficient; Half-value layer; Radiation shielding; BORATE GLASSES; LUMINESCENCE PROPERTIES; BOROSILICATE GLASSES; OPTICAL-ABSORPTION; RADIATION; ER3+; MULTICOMPONENT; EMISSION; LASER; BI2O3;
D O I
10.1016/j.radphyschem.2019.108633
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Tellurite-rich glasses containing Sm3+, Dy3+, and Er3+ ions with nominal chemical composition of 69 TeO2.10 Bi2O3-10 BaO-10 ZnO-1.0 Sm2O3/1.0 Dy2O3/1.0 Er2O3 (mol%) were fabricated. The gamma radiation attenuation features of the synthesized glasses were compared with two other tellurite glass systems with the chemical composition of 68 TeO2-(22-x) Bi2O3.10 ZnO. (x) PbO (x = 10, 12, 14, 16 and 18 mol%), and 75 TeO(2-)20 B(2)O(3-)5 MxOy (mol%) (MxOy = WO3, Nb2O5, PbO, Nd2O3, Y2O3). The mass attenuation coefficients (mu/.) (MAC) were computed from 0.015 MeV to 15 MeV photon energies using the XCOM program. Using the obtained mu/. values, effective atomic number (Z(eff)), electron density (N-e), half-value layer (HVL) and mean free path (MFP) were determined at different photon energies. The results clearly reveal that the MAC depends upon the heavy metals present in the studied glasses, and such addition increases the shielding capabilities of the samples against the gamma radiation. The Z(eff) and N-e confirmed the shielding effects with a variation in heavy metals content. The HVL and MFP values indicate the potential application in radiation insulation with less probability of interactions with gamma photons in the investigated tellurite glasses. It is found that the HVL or MFP values of the A. C glasses lies in between the HVL or MFP values of the S1 - S5 and the T1. T5 glasses, respectively. Thus, the synthesized glasses are better shielding materials than the T1 - T5 glasses and possess slightly less gamma-ray shielding capacity than that of S1-S5 glasses.
引用
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页数:14
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