Synthesis of controllable monodisperse gold nanoparticles using wood material and their catalytic activity for p-nitrophenol reduction

被引:8
作者
Lin, Xiaobo [1 ]
Wu, Min [2 ]
Kuga, Shigenori [2 ]
Endo, Takashi [3 ]
Huang, Yong [2 ]
机构
[1] Shijiazhuang Tiedao Univ, Hebei Prov Key Lab Traff Engn Mat, Shijiazhuang, Hebei, Peoples R China
[2] Chinese Acad Sci, Tech Inst Phys & Chem, 29 Zhongguancun East Rd, Beijing 100190, Peoples R China
[3] Natl Inst Adv Ind Sci & Technol, Res Inst Sustainable Chem, Hiroshima, Japan
基金
中国国家自然科学基金;
关键词
CULTURED SYCAMORE CELLS; SILVER NANOPARTICLES; STEP SYNTHESIS; SIZE; GREEN; NANOCLUSTERS; NANOCRYSTALS; PLATINUM; WALLS; MEDIA;
D O I
10.1038/pj.2016.51
中图分类号
O63 [高分子化学(高聚物)];
学科分类号
070305 ; 080501 ; 081704 ;
摘要
Monodisperse gold nanoparticles (Au NPs) with sizes between 2.3 and 23.1 nm were synthesized with the assistance of a natural wood material as a reductant/dispersant. The average diameter of the Au NPs could be controlled by varying the concentration of the Au precursor, and the size distribution could be improved by the addition of NaOH. The different growing processes of Au NPs with and without NaOH were comprehensively studied. The obtained wood-supported Au NPs showed high catalytic activity for the reduction of p-nitrophenol as a model reaction. Moreover, Au NPs with smaller sizes exhibited higher catalytic activity and the catalyst could be easily recovered via centrifugation for reuse.
引用
收藏
页码:919 / 923
页数:5
相关论文
共 29 条
[1]   STRUCTURE OF PLANT-CELL WALLS .2. HEMICELLULOSE OF WALLS OF SUSPENSION-CULTURED SYCAMORE CELLS [J].
BAUER, WD ;
TALMADGE, KW ;
KEEGSTRA, K ;
ALBERSHEIM, P .
PLANT PHYSIOLOGY, 1973, 51 (01) :174-187
[2]  
Chen L., 2015, J NANOSCI NANOTECHNO, V15, P2761
[3]   Radiolytic control of the size of colloidal gold nanoparticles [J].
Henglein, A ;
Meisel, D .
LANGMUIR, 1998, 14 (26) :7392-7396
[4]   A simple large-scale synthesis of nearly monodisperse gold and silver nanoparticles with adjustable sizes and with exchangeable surfactants [J].
Hiramatsu, H ;
Osterloh, FE .
CHEMISTRY OF MATERIALS, 2004, 16 (13) :2509-2511
[5]   One-step, size-controlled synthesis of gold nanoparticles at room temperature using plant tannin [J].
Huang, Xin ;
Wu, Hao ;
Liao, Xuepin ;
Shi, Bi .
GREEN CHEMISTRY, 2010, 12 (03) :395-399
[6]   Single-phase and gram-scale routes toward nearly monodisperse Au and other noble metal nanocrystals [J].
Jana, NR ;
Peng, XG .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2003, 125 (47) :14280-14281
[7]   Size control of gold nanocrystals in citrate reduction: The third role of citrate [J].
Ji, Xiaohui ;
Song, Xiangning ;
Li, Jun ;
Bai, Yubai ;
Yang, Wensheng ;
Peng, Xiaogang .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2007, 129 (45) :13939-13948
[8]   Aqueous-phase synthesis of monodisperse plasmonic gold nanocrystals using shortened single-walled carbon nanotubes [J].
Kim, Jin-Woo ;
Moon, Hyung-Mo ;
Benamara, Mourad ;
Sakon, Joshua ;
Salamo, Gregory J. ;
Zharov, Vladimir P. .
CHEMICAL COMMUNICATIONS, 2010, 46 (38) :7142-7144
[9]   One-Step Synthesis of Folic Acid Protected Gold Nanoparticles and Their Receptor-Mediated Intracellular Uptake [J].
Li, Gaiping ;
Li, Dan ;
Zhang, Lixue ;
Zhai, Junfeng ;
Wang, Erkang .
CHEMISTRY-A EUROPEAN JOURNAL, 2009, 15 (38) :9868-9873
[10]   Eco-friendly synthesis and antibacterial activity of silver nanoparticles reduced by nano-wood materials [J].
Lin, Xiaobo ;
Wang, Fengqi ;
Kuga, Shigenori ;
Endo, Takashi ;
Wu, Min ;
Wu, Dayong ;
Huang, Yong .
CELLULOSE, 2014, 21 (04) :2489-2496