Hydrogen Sulfide Capture: From Absorption in Polar Liquids to Oxide, Zeolite, and Metal-Organic Framework Adsorbents and Membranes

被引：515

作者：

Shah, Mansi S. ^{[1
]}

Tsapatsis, Michael ^{[1
]}

Siepmann, J. Ilja ^{[1
,2
,3
]}

机构：

[1] Univ Minnesota, Dept Chem Engn & Mat Sci, 421 Washington Ave SE, Minneapolis, MN 55455 USA

[2] Univ Minnesota, Dept Chem, 207 Pleasant St SE, Minneapolis, MN 55455 USA

[3] Univ Minnesota, Chem Theory Ctr, 207 Pleasant St SE, Minneapolis, MN 55455 USA

来源：

CHEMICAL REVIEWS | 2017年 / 117卷 / 14期

关键词：

TEMPERATURE H2S REMOVAL; MONTE-CARLO SIMULATIONS; CO2-SELECTIVE POLYMER MEMBRANES; ENHANCED REACTIVE ADSORPTION; DENSITY-FUNCTIONAL THEORY; GAS PERMEATION PROPERTIES; EUTECTIC SOLVENTS DESS; PROTIC IONIC LIQUIDS; QUALITY NATURAL-GAS; OF-THE-ART;

D O I：

10.1021/acs.chemrev.7b00095

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Hydrogen sulfide removal is a long-standing economic and environmental challenge faced by the oil and gas industries. H2S separation processes using reactive and non-reactive absorption and adsorption, membranes, and cryogenic distillation are reviewed. A detailed discussion is presented on new developments in adsorbents, such as ionic liquids, metal oxides, metals, metal organic frameworks, zeolites, carbon-based materials, and composite materials; and membrane technologies for H2S removal. This Review attempts to exhaustively compile the existing literature on sour gas sweetening and to identify promising areas for future developments in the field.

引用

页码：9755 / 9803

页数：49

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