Bright Multicolored Photoluminescence of Hybrid Graphene/Silicon Optoelectronics

被引：15
作者：
Liu, Ken [1 ]
Zhu, Zhi Hong [1 ]
Li, Xiu Jian [2 ]
Zhang, Jian Fa [1 ]
Yuan, Xiao Dong [1 ,3 ]
Guo, Chu Cai [1 ]
Xu, Wei [1 ]
Qin, Shi Qiao [1 ,3 ]
机构：
[1] Natl Univ Def Technol, Coll Optoelect Sci & Engn, Changsha 410073, Hunan, Peoples R China
[2] Natl Univ Def Technol, Coll Sci, Changsha 410073, Hunan, Peoples R China
[3] Natl Univ Def Technol, State Key Lab High Performance Comp, Changsha 410073, Hunan, Peoples R China
来源：
ACS PHOTONICS | 2015年 / 2卷 / 07期
基金：
中国国家自然科学基金;
关键词：
graphene; silicon; frequency-upconverted photoluminescence; broadband; hot carrier multiplication; hot carrier scattering; CARRIER MULTIPLICATION; SCATTERING; PHOTODETECTOR;
D O I：
10.1021/acsphotonics.5b00051
中图分类号：
TB3 [工程材料学];
学科分类号：
0805 ; 080502 ;
摘要：
Graphene does not possess a band gap, and hot carrier relaxation in graphene is an ultrafast processs. This leads to a very low emission efficiency of graphene. We demonstrate bright multicolored frequency-upconverted photoluminescence from graphene via three-photon absorption by femtosecond laser injection at a communication wavelength 1.57 mu m. The broadband and multiwavelength emission from graphene is based on the model of ultrafast electron-hole pair recombination and asymmetrical energized electron-hole radiation recombination in graphene. Furthermore, we show photoluminescence variation with blue light emission in the graphene/silicon hybrid system, with 2-3 orders of emission efficiency increase. The results demonstrate hot carrier multiplication and hot carrier scattering in graphene and could help to study the population inversion and broadband lasing of graphene.
引用
收藏
页码：797 / 804
页数：8
相关论文
共 30 条
  • [1] Ultrafast collinear scattering and carrier multiplication in graphene
    Brida, D.
    Tomadin, A.
    Manzoni, C.
    Kim, Y. J.
    Lombardo, A.
    Milana, S.
    Nair, R. R.
    Novoselov, K. S.
    Ferrari, A. C.
    Cerullo, G.
    Polini, M.
    [J]. NATURE COMMUNICATIONS, 2013, 4
  • [2] The electronic properties of graphene
    Castro Neto, A. H.
    Guinea, F.
    Peres, N. M. R.
    Novoselov, K. S.
    Geim, A. K.
    [J]. REVIEWS OF MODERN PHYSICS, 2009, 81 (01) : 109 - 162
  • [3] Controlling inelastic light scattering quantum pathways in graphene
    Chen, Chi-Fan
    Park, Cheol-Hwan
    Boudouris, Bryan W.
    Horng, Jason
    Geng, Baisong
    Girit, Caglar
    Zettl, Alex
    Crommie, Michael F.
    Segalman, Rachel A.
    Louie, Steven G.
    Wang, Feng
    [J]. NATURE, 2011, 471 (7340) : 617 - 620
  • [4] Cho CH, 2013, NAT PHOTONICS, V7, P285, DOI [10.1038/NPHOTON.2013.25, 10.1038/nphoton.2013.25]
  • [5] Coldren L. A., 1995, DIODE LASERS PHOTONI, p[126, 153]
  • [6] Monitoring dopants by Raman scattering in an electrochemically top-gated graphene transistor
    Das, A.
    Pisana, S.
    Chakraborty, B.
    Piscanec, S.
    Saha, S. K.
    Waghmare, U. V.
    Novoselov, K. S.
    Krishnamurthy, H. R.
    Geim, A. K.
    Ferrari, A. C.
    Sood, A. K.
    [J]. NATURE NANOTECHNOLOGY, 2008, 3 (04) : 210 - 215
  • [7] Electronic transport in two-dimensional graphene
    Das Sarma, S.
    Adam, Shaffique
    Hwang, E. H.
    Rossi, Enrico
    [J]. REVIEWS OF MODERN PHYSICS, 2011, 83 (02) : 407 - 470
  • [8] Chip-integrated ultrafast graphene photodetector with high responsivity
    Gan, Xuetao
    Shiue, Ren-Jye
    Gao, Yuanda
    Meric, Inanc
    Heinz, Tony F.
    Shepard, Kenneth
    Hone, James
    Assefa, Solomon
    Englund, Dirk
    [J]. NATURE PHOTONICS, 2013, 7 (11) : 883 - 887
  • [9] Gierz I, 2013, NAT MATER, V12, P1119, DOI [10.1038/NMAT3757, 10.1038/nmat3757]
  • [10] Regenerative oscillation and four-wave mixing in graphene optoelectronics
    Gu, T.
    Petrone, N.
    McMillan, J. F.
    van der Zande, A.
    Yu, M.
    Lo, G. Q.
    Kwong, D. L.
    Hone, J.
    Wong, C. W.
    [J]. NATURE PHOTONICS, 2012, 6 (08) : 554 - 559
123