Rapid phase-cycled two-dimensional optical spectroscopy in fluorescence and transmission mode

被引：60
|
作者：
Wagner, W
Li, CQ
Semmlow, J
Warren, WS
机构：
[1] Princeton Univ, Dept Elect Engn, Princeton, NJ 08544 USA
[2] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA
来源：
OPTICS EXPRESS | 2005年 / 13卷 / 10期
关键词：
D O I：
10.1364/OPEX.13.003697
中图分类号：
O43 [光学];
学科分类号：
070207 ; 0803 ;
摘要：
Two dimensional magnetic and optical spectra contain information about structure and dynamics inaccessible to the linear spectroscopist. Recently, phase cycling techniques in optical spectroscopy have extended the capabilities of two-dimensional electronic spectroscopy. Here, we present a method to generate collinear pump/probe pulses at high update rates for two-dimensional electronic spectroscopy. Both fluorescence mode and transmission mode photon echo data from rubidium vapor is presented. (C) 2005 Optical Society of America.
引用
收藏
页码：3697 / 3706
页数：10
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