A simple merocyanine tandem solar cell with extraordinarily high open-circuit voltage

被引:15
作者
Steinmann, V. [1 ]
Kronenberg, N. M. [1 ]
Lenze, M. R. [1 ]
Graf, S. M. [1 ]
Hertel, D. [1 ]
Buerckstuemmer, H. [2 ,3 ]
Wuerthner, F. [2 ,3 ]
Meerholz, K. [1 ]
机构
[1] Univ Cologne, Dept Chem, D-50939 Cologne, Germany
[2] Univ Wurzburg, Inst Organ Chem, D-97074 Wurzburg, Germany
[3] Univ Wurzburg, Rontgen Res Ctr Complex Mat Syst, D-97074 Wurzburg, Germany
关键词
PERFORMANCE; EFFICIENCY; DYES;
D O I
10.1063/1.3657145
中图分类号
O59 [应用物理学];
学科分类号
摘要
We present a highly efficient tandem solar cell based on a merocyanine dye, containing two identical subcells connected in series. A recombination layer of Al/MoO(3) was used. Due to a substantial improvement of the fill factor, the overall efficiency of the tandem cell was even higher than that of the single-cell reference with identical active layer thickness. By combining the planar heterojunction and the bulk heterojunction concept, efficiencies up to 4.8% were achieved while maintaining a rather simple, fully vacuum-processed device stack consisting of only four organic layers. The optimized open-circuit voltage was as large as 2.1V. (C) 2011 American Institute of Physics. [doi: 10.1063/1.3657145]
引用
收藏
页数:3
相关论文
共 20 条
[1]   Organic tandem solar cells: A review [J].
Ameri, Tayebeh ;
Dennler, Gilles ;
Lungenschmied, Christoph ;
Brabec, Christoph J. .
ENERGY & ENVIRONMENTAL SCIENCE, 2009, 2 (04) :347-363
[2]   Tailored merocyanine dyes for solution-processed BHJ solar cells [J].
Buerckstuemmer, Hannah ;
Kronenberg, Nils Michael ;
Gsaenger, Marcel ;
Stolte, Matthias ;
Meerholz, Klaus ;
Wuerthner, Frank .
JOURNAL OF MATERIALS CHEMISTRY, 2010, 20 (02) :240-243
[3]   Dicyanovinyl-Substituted Oligothiophenes: Structure-Property Relationships and Application in Vacuum-Processed Small-Molecule Organic Solar Cells [J].
Fitzner, Roland ;
Reinold, Egon ;
Mishra, Amaresh ;
Mena-Osteritz, Elena ;
Ziehlke, Hannah ;
Koerner, Christian ;
Leo, Karl ;
Riede, Moritz ;
Weil, Matthias ;
Tsaryova, Olga ;
Weiss, Andre ;
Uhrich, Christian ;
Pfeiffer, Martin ;
Baeuerle, Peter .
ADVANCED FUNCTIONAL MATERIALS, 2011, 21 (05) :897-910
[4]  
Frohne H, 2002, CHEMPHYSCHEM, V3, P795, DOI 10.1002/1439-7641(20020916)3:9<795::AID-CPHC795>3.0.CO
[5]  
2-A
[6]   Device operation of organic tandem solar cells [J].
Hadipour, A. ;
de Boer, B. ;
Blom, P. W. M. .
ORGANIC ELECTRONICS, 2008, 9 (05) :617-624
[7]   Simultaneous Enhancement of Open-Circuit Voltage, Short-Circuit Current Density, and Fill Factor in Polymer Solar Cells [J].
He, Zhicai ;
Zhong, Chengmei ;
Huang, Xun ;
Wong, Wai-Yeung ;
Wu, Hongbin ;
Chen, Liwei ;
Su, Shijian ;
Cao, Yong .
ADVANCED MATERIALS, 2011, 23 (40) :4636-+
[8]   Direct Comparison of Highly Efficient Solution- and Vacuum-Processed Organic Solar Cells Based on Merocyanine Dyes [J].
Kronenberg, Nils M. ;
Steinmann, Vera ;
Buerckstuemmer, Hannah ;
Hwang, Jaehyung ;
Hertel, Dirk ;
Wuerthner, Frank ;
Meerholz, Klaus .
ADVANCED MATERIALS, 2010, 22 (37) :4193-+
[9]   Bulk heterojunction organic solar cells based on merocyanine colorants [J].
Kronenberg, Nils M. ;
Deppisch, Manuela ;
Wuerthner, Frank ;
Lademann, Hans W. A. ;
Deing, Kaja ;
Meerholz, Klaus .
CHEMICAL COMMUNICATIONS, 2008, (48) :6489-6491
[10]   For the Bright Future-Bulk Heterojunction Polymer Solar Cells with Power Conversion Efficiency of 7.4% [J].
Liang, Yongye ;
Xu, Zheng ;
Xia, Jiangbin ;
Tsai, Szu-Ting ;
Wu, Yue ;
Li, Gang ;
Ray, Claire ;
Yu, Luping .
ADVANCED MATERIALS, 2010, 22 (20) :E135-+