Recent advances towards aqueous hydrogen peroxide formation in a direct current plasma-liquid system

被引：16

作者：

Chen, Qiang ^{[1
,4
]}

Li, Junshuai ^{[2
,3
]}

Chen, Qiang ^{[1
,4
]}

Ostrikov, Kostya ^{[5
,6
]}

机构：

[1] Xiamen Univ, Fujian Prov Key Lab Plasma & Magnet Resonance, Key Lab Electromagnet Wave Sci & Detect Technol, Shenzhen Res Inst,Inst Electromagnet & Acoust, Xiamen 361005, Peoples R China

[2] Lanzhou Univ, LONGi Inst Future Technol, Lanzhou, Peoples R China

[3] Lanzhou Univ, Sch Mat & Energy, Lanzhou, Peoples R China

[4] Beijing Inst Graph Commun, Lab Plasma Phys & Mat, Beijing, Peoples R China

[5] Queensland Univ Technol QUT, Sch Chem & Phys, Brisbane, Qld, Australia

[6] Queensland Univ Technol QUT, QUT Ctr Mat Sci, Brisbane, Qld, Australia

来源：

HIGH VOLTAGE | 2022年 / 7卷 / 03期

基金：

澳大利亚研究理事会; 中国国家自然科学基金;

关键词：

GLOW-DISCHARGE ELECTROLYSIS; OPTICAL-EMISSION; HYDROXYL RADICALS; GAS-PHASE; PHOTOCHEMICAL OXIDATION; INTERFACIAL REACTIONS; WATER; H2O2; DEGRADATION; IONS;

D O I：

10.1049/hve2.12189

中图分类号：

TM [电工技术]; TN [电子技术、通信技术];

学科分类号：

0808 ; 0809 ;

摘要：

The aqueous phase hydrogen peroxide (H2O2aq) produced from the plasma-liquid interactions can directly or synergistically (with other substances) affect the liquid chemistry, and therefore it is important to unfold the H(2)O(2aq )formation mechanism. However, up to now, a consensus on the H2O2aq formation mechanism is not reached. This review aims to survey the recent advances on the understanding of the H2O2aq formation mechanism in the system of a direct current discharge plasma operated over a liquid electrode. Theoretical and experimental analyses indicate that the recombination of dissolved OH radicals (OHaq) is the dominant process for the H(2)O(2aq )formation, while the purported plasma-induced photolysis of water and the dissolution of gaseous H2O2 are ruled out.

引用

页码：405 / 419

页数：15

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