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A novel ternary MoS2/MoO3/TiO2 composite for fast photocatalytic degradation of rhodamine B under visible-light irradiation
被引:23
作者:
Li, Zhenyu
[1
]
Cao, Fa
[1
]
Wang, Lei
[1
]
Chen, Zhiwu
[1
]
Ji, Xiaohong
[1
]
机构:
[1] South China Univ Technol, Sch Mat Sci & Engn, Guangzhou 510641, Guangdong, Peoples R China
基金:
中国国家自然科学基金;
关键词:
MOS2;
NANOSHEETS;
NANOPARTICLES;
NANOBELTS;
GRAPHENE;
D O I:
10.1039/c9nj04107a
中图分类号:
O6 [化学];
学科分类号:
0703 ;
摘要:
In this article, novel ternary MoS2/MoO3/TiO2 composite catalysts were developed. The photocatalytic performance of the ternary MoS2/MoO3/TiO2 composites was evaluated by photo-degradation of rhodamine B (RhB). It was found that the photocatalytic ability of the composites was strongly dependent on the mass ratio of MoS2-MoO3 to MoS2-MoO3-TiO2. The ternary composite catalyst with optimum composition showed a fast degradation rate (maximum similar to 0.138 min(-1)), which could degrade over 95% of RhB solution (10 mg L-1) within 20 min under visible light (lambda > 420 nm) irradiation. The possible photocatalytic mechanism was proposed based on the trapping photocatalytic experiment and band alignment of the composite. The synergistic effect of the strong absorption of the catalyst and the efficient separation of photogenerated electron-hole pairs by the novel ternary composite contributed to the enhanced photocatalytic activity.
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页码:537 / 542
页数:6
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