A novel ternary MoS2/MoO3/TiO2 composite for fast photocatalytic degradation of rhodamine B under visible-light irradiation

被引:23
作者
Li, Zhenyu [1 ]
Cao, Fa [1 ]
Wang, Lei [1 ]
Chen, Zhiwu [1 ]
Ji, Xiaohong [1 ]
机构
[1] South China Univ Technol, Sch Mat Sci & Engn, Guangzhou 510641, Guangdong, Peoples R China
基金
中国国家自然科学基金;
关键词
MOS2; NANOSHEETS; NANOPARTICLES; NANOBELTS; GRAPHENE;
D O I
10.1039/c9nj04107a
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
In this article, novel ternary MoS2/MoO3/TiO2 composite catalysts were developed. The photocatalytic performance of the ternary MoS2/MoO3/TiO2 composites was evaluated by photo-degradation of rhodamine B (RhB). It was found that the photocatalytic ability of the composites was strongly dependent on the mass ratio of MoS2-MoO3 to MoS2-MoO3-TiO2. The ternary composite catalyst with optimum composition showed a fast degradation rate (maximum similar to 0.138 min(-1)), which could degrade over 95% of RhB solution (10 mg L-1) within 20 min under visible light (lambda > 420 nm) irradiation. The possible photocatalytic mechanism was proposed based on the trapping photocatalytic experiment and band alignment of the composite. The synergistic effect of the strong absorption of the catalyst and the efficient separation of photogenerated electron-hole pairs by the novel ternary composite contributed to the enhanced photocatalytic activity.
引用
收藏
页码:537 / 542
页数:6
相关论文
共 50 条
  • [21] The MoS2/TiO2 heterojunction composites with enhanced activity for CO2 photocatalytic reduction under visible light irradiation
    Jia, Peng-Yao
    Guo, Rui-tang
    Pan, Wei-guo
    Huang, Chun-ying
    Tang, Jun-ying
    Liu, Xing-yu
    Qin, Hao
    Xu, Qi-yan
    COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS, 2019, 570 : 306 - 316
  • [22] Morphology-controlled synthesis of TiO2/MoS2 nanocomposites with enhanced visible-light photocatalytic activity
    Sun, Yuanqing
    Lin, Huihui
    Wang, Chuanxi
    Wu, Qian
    Wang, Xiaojie
    Yang, Minghui
    INORGANIC CHEMISTRY FRONTIERS, 2018, 5 (01): : 145 - 152
  • [23] PHOTOCATALYTIC DEGRADATION OF ORGANIC POLLUTANTS WITH PT-CaFe2O4/TiO2 COMPOSITE UNDER VISIBLE-LIGHT IRRADIATION
    Ojha, D. P.
    Karki, H. P.
    Song, J. H.
    Kim, H. J.
    DIGEST JOURNAL OF NANOMATERIALS AND BIOSTRUCTURES, 2018, 13 (03) : 631 - 639
  • [24] Three-dimensional MoO3 nanoflowers assembled with nanosheets for rhodamine B degradation under visible light
    Huang, Licheng
    Fang, Wencheng
    Yang, Ying
    Wu, Jie
    Yu, Hui
    Dong, Xiangting
    Wang, Tingting
    Liu, Zhelin
    Zhao, Bo
    MATERIALS RESEARCH BULLETIN, 2018, 108 : 38 - 45
  • [25] Enhancement of photocatalytic property on ZnS/MoS2 composite under visible light irradiation
    Cheng, Jiushan
    Han, Lu
    Wei, Yen
    Chen, Qiang
    2017 INTERNATIONAL CONFERENCE ON MECHANICAL, AERONAUTICAL AND AUTOMOTIVE ENGINEERING (ICMAA 2017), 2017, 108
  • [26] Fabrication of TiO2/MoS2@zeolite photocatalyst and its photocatalytic activity for degradation of methyl orange under visible light
    Zhang, Weiping
    Xiao, Xinyan
    Zheng, Lili
    Wan, Caixia
    APPLIED SURFACE SCIENCE, 2015, 358 : 468 - 478
  • [27] MoS2 nanosheet/TiO2 nanowire hybrid nanostructures for enhanced visible-light photocatalytic activities
    Shen, Meng
    Yan, Zhiping
    Yang, Lei
    Du, Pingwu
    Zhang, Jingyu
    Xiang, Bin
    CHEMICAL COMMUNICATIONS, 2014, 50 (97) : 15447 - 15449
  • [28] Photodegradation of Rhodamine B on Sulfur Doped ZnO/TiO2 Nanocomposite Photocatalyst under Visible-light Irradiation
    Guo Jianfeng
    Li Jingxia
    Yin Anyuan
    Fan Kangnian
    Dai Weilin
    CHINESE JOURNAL OF CHEMISTRY, 2010, 28 (11) : 2144 - 2150
  • [29] Photocatalytic Performance of SiO2/CNOs/TiO2 to Accelerate the Degradation of Rhodamine B under Visible Light
    Zhang, Weike
    Zhang, Yanrong
    Yang, Kai
    Yang, Yanqing
    Jia, Jia
    Guo, Lijun
    NANOMATERIALS, 2019, 9 (12)
  • [30] Photoelectrocatalytic degradation of sulfadiazine by Ag3PO4/MoS2/TiO2 nanotube array electrode under visible light irradiation
    Teng, Wei
    Xu, Jin
    Cui, Yanjuan
    Yu, Jiuheng
    JOURNAL OF ELECTROANALYTICAL CHEMISTRY, 2020, 868 (868)