Treatment of zeolite adsorbed material as a potential nuclear waste glass-ceramic matrix

被引:8
作者
Wei, Guilin [1 ]
Luo, Fen [1 ]
Miao, Yulong [1 ]
Han, Wenhong [1 ]
Xie, Yi [2 ]
Huang, Wenxiao [3 ]
Xu, Zhengfan [3 ]
Lu, Xirui [1 ,4 ,5 ]
机构
[1] Southwest Univ Sci & Technol, State Key Lab Environm Friendly Energy Mat, Mianyang, Sichuan, Peoples R China
[2] Tsinghua Univ, Collahorat Innovat Ctr Adv Nucl Energy Technol, Inst Nucl & New Energy Technol, Beijing, Peoples R China
[3] Guangdong Prov Key Lab Radioact & Rare Resource U, Shaoguan, Peoples R China
[4] Southwest Univ Sci & Technol, Fundamental Sci Nucl Wastes & Environm Safety Lab, Mianyang, Sichuan, Peoples R China
[5] Southwest Univ Sci & Technol, Collaborat Innovat Ctr Nucl Wastes & Environm Saf, Mianyang, Sichuan, Peoples R China
关键词
glass-ceramics; nuclear waste; treatment conditions; zeolite; SILICA-GEL; IMMOBILIZATION; IODINE; REMOVAL; ADSORPTION; CESIUM;
D O I
10.1111/jace.18094
中图分类号
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Zeolite, as a common adsorption material, should be safely treated after adsorbing different nuclear wastes. In this study, different types of simulated zeolite wastes were successfully immobilized based on the exploring result of suitable experiment conditions. Firstly, sintering temperature was selected based on TG-DSC and phase results, which represented mainly as glassy phase. Then, the holding time was chosen through density and Vickers hardness results. For the sintering of zeolite, the suitable temperature is 1500celcius and the holding time is 1 h. Through the fitting process, FT-IR results demonstrate that the main microstructures compose of sheet silicates. Three types of simulated zeolite wastes can successfully transform into matrix and all the waste contents were uniformly immobilized. Finally, SEM-EDS results prove that the matrix is glass-ceramic which can well immobilize the considered nuclear wastes. This work proposes the idea of treatment of zeolite adsorbed material as a potential nuclear waste glass-ceramic matrix and the suitable conditions were also investigated.
引用
收藏
页码:257 / 267
页数:11
相关论文
共 34 条
[1]   Effect of concentration on hydrodynamic size of magnetite-based ferrofluid as a potential MRI contrast agent [J].
Ahmadi, Reza ;
Hosseini, Hamid Reza Madaah ;
Masoudi, Afshin ;
Omid, Hamed ;
Namivandi-Zangeneh, Rashin ;
Ahmadi, Maryam ;
Ahmadi, Zahra ;
Gu, Ning .
COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS, 2013, 424 :113-117
[2]   Drug delivery system for an anticancer agent, chlorogenate-Zn/Al-layered double hydroxide nanohybrid synthesised using direct co-precipitation and ion exchange methods [J].
Barahuie, Farahnaz ;
Hussein, Mohd Zobir ;
Arulselvan, Palanisamy ;
Fakurazi, Sharida ;
Zainal, Zulkarnain .
JOURNAL OF SOLID STATE CHEMISTRY, 2014, 217 :31-41
[3]  
Bock J., 1970, Journal of the American Ceramic Society, V53, P69, DOI 10.1111/j.1151-2916.1970.tb12012.x
[4]   Microwave vitrification of uranium-contaminated soil for nuclear test site and chemical stability [J].
Chen, Shunzhang ;
Shu, Xiaoyan ;
Tang, Hexi ;
Mao, Xueli ;
Xu, Chen ;
Lu, Xirui .
CERAMICS INTERNATIONAL, 2019, 45 (10) :13334-13339
[5]   INTERPRETATION OF RAMAN DIFFUSION SPECTRA OF BINARY SILICA GLASSES [J].
ETCHEPARE, J .
SPECTROCHIMICA ACTA PART A-MOLECULAR SPECTROSCOPY, 1970, A 26 (11) :2147-+
[6]   Adsorption of radioactive iodide by natural zeolites [J].
Faghihian, H ;
Maragheh, MG ;
Malekpour, A .
JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY, 2002, 254 (03) :545-550
[7]   Ammonium removal from aqueous solutions by using natural Chinese (Chende) zeolite as adsorbent [J].
Huang, Haiming ;
Xiao, Xianming ;
Yan, Bo ;
Yang, Liping .
JOURNAL OF HAZARDOUS MATERIALS, 2010, 175 (1-3) :247-252
[8]   Development of silver nanoparticle-doped adsorbents for the separation and recovery of radioactive iodine from alkaline solutions [J].
Kim, Taewoon ;
Lee, Seung-Kon ;
Lee, Suseung ;
Lee, Jun Sig ;
Kim, Sang Wook .
APPLIED RADIATION AND ISOTOPES, 2017, 129 :215-221
[9]   Vitrification processes of simulated cesium sorbing zeolite waste [J].
Kimura, Ryou ;
Inagaki, Yaohiro ;
Idemitsu, Kazuya ;
Arima, Tatsumi .
PROGRESS IN NUCLEAR ENERGY, 2018, 108 :497-502
[10]   Ammonium removal from aqueous solutions using microwave-treated natural Chinese zeolite [J].
Lei, Lecheng ;
Li, Xiaojuan ;
Zhang, Xingwang .
SEPARATION AND PURIFICATION TECHNOLOGY, 2008, 58 (03) :359-366