Characteristics of Inorganic-Organic Hybrid Membranes Containing Carbon Nanotubes with Increased Iron-Encapsulated Content for CO2 Separation

被引：2
作者：
Rybak, Aleksandra [1 ]
Rybak, Aurelia [2 ]
Kaszuwara, Waldemar [3 ]
Boncel, Slawomir [1 ]
Kolanowska, Anna [1 ]
Kolev, Spas D. [4 ]
机构：
[1] Silesian Tech Univ, Fac Chem, Strzody 7, PL-44100 Gliwice, Poland
[2] Silesian Tech Univ, Fac Min Safety Engn & Ind Automat, PL-44100 Gliwice, Poland
[3] Warsaw Univ Technol, Fac Mat Sci & Engn, PL-00661 Warsaw, Poland
[4] Univ Melbourne, Sch Chem, Parkville, Vic 3010, Australia
来源：
MEMBRANES | 2022年 / 12卷 / 02期
关键词：
CO2; separation; inorganic-organic hybrid membranes; mechanical properties; magnetic measurements; thermal analysis; MIXED MATRIX MEMBRANES; POLY(PHENYLENE OXIDE) MEMBRANES; GAS-TRANSPORT PROPERTIES; MECHANICAL-PROPERTIES; COMPOSITE MEMBRANES; HYPERBRANCHED POLYIMIDE; POLYMER MATRICES; SILICA; PERMEATION; EFFICIENT;
D O I：
10.3390/membranes12020132
中图分类号：
Q5 [生物化学]; Q7 [分子生物学];
学科分类号：
071010 ; 081704 ;
摘要：
Novel inorganic-organic hybrid membranes Fe@MWCNT/PPO or Fe@MWCNT-OH/SPPO (with a new type of CNTs characterized by increased iron content 5.80 wt%) were synthesized for CO<INF>2</INF> separation. The introduction of nanofillers into the polymer matrix has significantly improved the hybrid membrane's gas transport (D, P, S, and alpha<INF>CO<INF>2</INF>/N<INF>2</INF></INF>), magnetic, thermal, and mechanical parameters. It was found that magnetic casting has improved the alignment and dispersion of Fe@MWCNTs. At the same time, CNTs and polymer chemical modification enhanced interphase compatibility and the membrane's CO<INF>2</INF> separation efficiency. The thermo-oxidative stability and mechanical and magnetic parameters of composites were improved by increasing new CNTs loading. Cherazi's model turned out to be suitable for describing the CO<INF>2</INF> transport through analyzed hybrid membranes.
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页数：20
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