A comprehensive review on reactive oxygen species (ROS) in advanced oxidation processes (AOPs)

被引:216
作者
Dong, Chencheng [1 ,2 ,4 ]
Fang, Wenzhang [3 ]
Yi, Qiuying [5 ]
Zhang, Jinlong [1 ,2 ]
机构
[1] East China Univ Sci & Technol, Sch Chem & Mol Engn, Shanghai Engn Res Ctr Multimedia Environm Catalysi, Key Lab Adv Mat, 130 Meilong Rd, Shanghai 200237, Peoples R China
[2] East China Univ Sci & Technol, Inst Fine Chem, Shanghai Engn Res Ctr Multimedia Environm Catalysi, Sch Chem & Mol Engn, 130 Meilong Rd, Shanghai 200237, Peoples R China
[3] Zhejiang Univ, Dept Polymer Sci & Engn, MOE Key Lab Macromol Synth & Functionalizat, Hangzhou, Peoples R China
[4] Univ Hong Kong, Dept Civil Engn, Hong Kong, Peoples R China
[5] Tongji Univ, Shanghai Inst Pollut Control & Ecol Secur, Sch Environm Sci & Engn, State Key Lab Pollut Control & Resource Reuse, Shanghai 200092, Peoples R China
基金
中国国家自然科学基金;
关键词
AOP; Fenton; ROS; PMS; Singlet oxygen; ELECTRO-FENTON PROCESS; STOBER-LIKE METHOD; PHOTO-FENTON; ORGANIC POLLUTANTS; H2O2; GENERATION; GRAPHENE-OXIDE; WASTE-WATER; PEROXYMONOSULFATE ACTIVATION; CATALYTIC-OXIDATION; FE3O4; NANOPARTICLES;
D O I
10.1016/j.chemosphere.2022.136205
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In this account, the reactive oxygen species (ROS) were comprehensively reviewed, which were based on electro-Fenton and photo-Fenton processes and correlative membrane filtration technology. Specifically, this review focuses on the fundamental principles and applications of advanced oxidation processes (AOPs) based on a series of nanomaterials, and we compare the pros and cons of each method and point out the perspective. Further, the emerging reviews regarding AOPs rarely emphasize the involved ROS and consider the convenience of radical classification and transformation mechanism, such a review is of paramount importance to be needed. Owing to the strong oxidation ability of radical (e.g., center dot OH, O-2(center dot-), and SO4 center dot-) and non-radical (e.g., (1)O(2 )and H2O2), these ROS would attack the organic contaminants of emerging concern, thus achieving the goal of environmental reme-diation. Hopefully, this review can offer detailed theoretical guidance for the researchers, and we believe it able to offer the frontier knowledge of AOPs for wastewater treatment plants (WWTPs).
引用
收藏
页数:18
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