Magnetic excitations in the ground state of Yb2Ti2O7

被引:14
作者
Pecanha-Antonio, Viviane [1 ,2 ]
Feng, Erxi [1 ]
Su, Yixi [1 ]
Pomjakushin, Vladimir [3 ]
Demmel, Franz [4 ]
Chang, Lieh-Jeng [5 ]
Aldus, Robert J. [1 ]
Xiao, Yinguo [6 ,7 ]
Lees, Martin R. [8 ]
Bruckel, Thomas [1 ,6 ,7 ]
机构
[1] Forschungszentrum Julich GmbH, Heinz Maier Leibnitz Zentrum MLZ, JCNS, Lichtenbergstr 1, D-85747 Garching, Germany
[2] Tech Univ Munich, Phys Dept, D-85747 Garching, Germany
[3] Paul Scherrer Inst, Lab Neutron Scattering & Imaging LNS, CH-5232 Villigen, Switzerland
[4] Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England
[5] Natl Cheng Kung Univ, Dept Phys, Tainan 70101, Taiwan
[6] Forschungszentrum Julich GmbH, JCNS, D-52425 Julich, Germany
[7] Forschungszentrum Julich GmbH, PGI, D-52425 Julich, Germany
[8] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England
基金
英国科学技术设施理事会;
关键词
PYROCHLORES; OXIDES; FIELD;
D O I
10.1103/PhysRevB.96.214415
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We report an extensive study on the zero field ground state of a powder sample of the pyrochlore Yb2Ti2O7. A sharp heat capacity anomaly that labels a low temperature phase transition in this material is observed at 280 mK. Neutron diffraction shows that a quasicollinear ferromagnetic order develops below Tc with a magnetic moment of 0.87(2)mu B. High resolution inelastic neutron scattering measurements show, belowthe phase transition temperature, sharp gapped low-lying magnetic excitations coexisting with a remnant quasielastic contribution likely associated with persistent spin fluctuations. Moreover, a broad inelastic continuum of excitations at similar to 0.6 meV is observed from the lowest measured temperature up to at least 2.5 K. At 10 K, the continuum has vanished and a broad quasielastic conventional paramagnetic scattering takes place at the observed energy range. Finally, we show that the exchange parameters obtained within the framework of linear spin-wave theory do not accurately describe the observed zero field inelastic neutron scattering data.
引用
收藏
页数:11
相关论文
共 40 条
  • [1] Vindication of Yb2Ti2O7 as a Model Exchange Quantum Spin Ice
    Applegate, R.
    Hayre, N. R.
    Singh, R. R. P.
    Lin, T.
    Day, A. G. R.
    Gingras, M. J. P.
    [J]. PHYSICAL REVIEW LETTERS, 2012, 109 (09)
  • [2] Impact of stoichiometry of Yb2Ti2O7 on its physical properties
    Arpino, K. E.
    Trump, B. A.
    Scheie, A. O.
    McQueen, T. M.
    Koohpayeh, S. M.
    [J]. PHYSICAL REVIEW B, 2017, 95 (09)
  • [3] HEAT-CAPACITY MEASUREMENTS ON RARE-EARTH DOUBLE OXIDES R2M2O7
    BLOTE, HWJ
    WIELINGA, RF
    HUISKAMP, WJ
    [J]. PHYSICA, 1969, 43 (04): : 549 - &
  • [4] Higgs transition from a magnetic Coulomb liquid to a ferromagnet in Yb2Ti2O7
    Chang, Lieh-Jeng
    Onoda, Shigeki
    Su, Yixi
    Kao, Ying-Jer
    Tsuei, Ku-Ding
    Yasui, Yukio
    Kakurai, Kazuhisa
    Lees, Martin Richard
    [J]. NATURE COMMUNICATIONS, 2012, 3
  • [5] Yb2Sn2O7: A magnetic Coulomb liquid at a quantum critical point
    Dun, Z. L.
    Choi, E. S.
    Zhou, H. D.
    Hallas, A. M.
    Silverstein, H. J.
    Qiu, Y.
    Copley, J. R. D.
    Gardner, J. S.
    Wiebe, C. R.
    [J]. PHYSICAL REVIEW B, 2013, 87 (13)
  • [6] High-resolution powder diffractometer HRPT for thermal neutrons at SINQ
    Fischer, P
    Frey, G
    Koch, M
    Könnecke, M
    Pomjakushin, V
    Schefer, J
    Thut, R
    Schlumpf, N
    Bürge, R
    Greuter, U
    Bondt, S
    Berruyer, E
    [J]. PHYSICA B, 2000, 276 : 146 - 147
  • [7] Magnetic pyrochlore oxides
    Gardner, Jason S.
    Gingras, Michel J. P.
    Greedan, John E.
    [J]. REVIEWS OF MODERN PHYSICS, 2010, 82 (01) : 53 - 107
  • [8] Spin-spin correlations in Yb2Ti2O7:: A polarized neutron scattering study -: art. no. 180404
    Gardner, JS
    Ehlers, G
    Rosov, N
    Erwin, RW
    Petrovic, C
    [J]. PHYSICAL REVIEW B, 2004, 70 (18): : 1 - 4
  • [9] Gapless quantum excitations from an icelike splayed ferromagnetic ground state in stoichiometric Yb2Ti2O7
    Gaudet, J.
    Ross, K. A.
    Kermarrec, E.
    Butch, N. P.
    Ehlers, G.
    Dabkowska, H. A.
    Gaulin, B. D.
    [J]. PHYSICAL REVIEW B, 2016, 93 (06)
  • [10] Neutron spectroscopic study of crystalline electric field excitations in stoichiometric and lightly stuffed Yb2Ti2O7
    Gaudet, J.
    Maharaj, D. D.
    Sala, G.
    Kermarrec, E.
    Ross, K. A.
    Dabkowska, H. A.
    Kolesnikov, A. I.
    Granroth, G. E.
    Gaulin, B. D.
    [J]. PHYSICAL REVIEW B, 2015, 92 (13)