Fabrication and enhanced photocatalytic properties of novel 3D MoS2/Na0.9Mg0.45Ti3.55O8 heterostructures

被引:5
作者
Lei, Yu-Xi [1 ,2 ]
Wang, Jing-Zhou [1 ]
Zhou, Jian-Ping [1 ]
Guo, Ze-Qing [1 ]
Ul Hassan, Qadeer [1 ]
机构
[1] Shaanxi Normal Univ, Sch Phys & Informat Technol, Xian 710119, Shaanxi, Peoples R China
[2] North Minzu Univ, Sch Elect & Informat Engn, Yinchuan 750021, Peoples R China
基金
中国国家自然科学基金;
关键词
MoS2; nanosheets; NMTO nanoplates; MoS2/NMTO heterostructure; Photocatalytic properties; MOS2; NANOSHEETS; TIO2; SEMICONDUCTOR; GRAPHENE; MECHANISM; SHEETS;
D O I
10.1016/j.apsusc.2017.08.169
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A novel three-dimensional (3D) nanocomposite based on Na0.9Mg0.45Ti3.55O8 (NMTO) nanoplates and few layered MoS2 nanosheets was fabricated via a facile two-step hydrothermal process. The few-layer MoS2 nanosheets were uniformly loaded on NMTO nanoplates to form a 3D hierarchical structure. The as-obtained MoS2/NMTO composites exhibit superior photocatalytic activities for stably photodegradating methylene blue (MB) and methyl orange (MO) in comparison with pure MoS2 nanoflowers and pure NMTO nanoplates. Importantly, the MoS2/NMTO heterostructure with 30 wt% of MoS2 shows the highest performance in photocatalytic degradation of dye molecules. The formation of 3D hierarchical heterostructure between few-layer MoS2 nanosheets and NMTO nanoplate favors the separation of photoinduced electron-hole pairs and contributes to the enhanced photocatalytic properties. (C) 2017 Elsevier B.V. All rights reserved.
引用
收藏
页码:733 / 741
页数:9
相关论文
共 43 条
[1]   Facile synthesis of ZnO flowers modified graphene like MoS2 sheets for enhanced visible-light-driven photocatalytic activity and antibacterial properties [J].
Awasthi, Ganesh Prasad ;
Adhikari, Surya Prasad ;
Ko, Sungwon ;
Kim, Han Joo ;
Park, Chan Hee ;
Kim, Cheol Sang .
JOURNAL OF ALLOYS AND COMPOUNDS, 2016, 682 :208-215
[2]   Mesoporous CuO-ZnO p-n heterojunction based nanocomposites with high specific surface area for enhanced photocatalysis and electrochemical sensing [J].
Chabri, Sumit ;
Dhara, Arnab ;
Show, Bibhutibhushan ;
Adak, Deepanjana ;
Sinha, Arijit ;
Mukherjee, Nillohit .
CATALYSIS SCIENCE & TECHNOLOGY, 2016, 6 (09) :3238-3252
[3]   Graphene-like MoS2/amorphous carbon composites with high capacity and excellent stability as anode materials for lithium ion batteries [J].
Chang, Kun ;
Chen, Weixiang ;
Ma, Lin ;
Li, Hui ;
Li, He ;
Huang, Feihe ;
Xu, Zhude ;
Zhang, Qingbo ;
Lee, Jim-Yang .
JOURNAL OF MATERIALS CHEMISTRY, 2011, 21 (17) :6251-6257
[4]   ELECTROCHEMICAL PHOTOLYSIS OF WATER AT A SEMICONDUCTOR ELECTRODE [J].
FUJISHIMA, A ;
HONDA, K .
NATURE, 1972, 238 (5358) :37-+
[5]   Interface role in the enhanced photocatalytic activity of TiO2-Na0.9Mg0.45Ti3.55O8 nanoheterojunction [J].
Guo, Ze-Qing ;
Zhou, Jian-Ping ;
Wang, Jing-Zhou ;
Hassan, Qadeer Ul ;
Yang, Jia ;
Ma, Yi .
APL MATERIALS, 2017, 5 (02)
[6]   A new-type of semiconductor Na0.9Mg0.45Ti3.55O8: preparation, characterization and photocatalysis [J].
Guo, Ze-Qing ;
Zhou, Jian-Ping ;
An, Long-Liang ;
Jiang, Jia-Xing ;
Zhu, Gang-Qiang ;
Deng, Chao-Yong .
JOURNAL OF MATERIALS CHEMISTRY A, 2014, 2 (47) :20358-20366
[7]   Preparation and photocatalytic behavior of MoS2 and WS2 nanocluster sensitized TiO2 [J].
Ho, WK ;
Yu, JC ;
Lin, J ;
Yu, JG ;
Li, PS .
LANGMUIR, 2004, 20 (14) :5865-5869
[8]   Metal-Semiconductor Heteronanocrystals with Desired Configurations for Plasmonic Photocatalysis [J].
Hong, Jong Wook ;
Wi, Dae Han ;
Lee, Su-Un ;
Han, Sang Woo .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2016, 138 (48) :15766-15773
[9]   Fabrication of 3D Hierarchical MoS2/Polyaniline and MoS2/C Architectures for Lithium-Ion Battery Applications [J].
Hu, Lianren ;
Ren, Yumei ;
Yang, Hongxia ;
Xu, Qun .
ACS APPLIED MATERIALS & INTERFACES, 2014, 6 (16) :14644-14652
[10]   Role of active oxygen species in the liquid-phase photocatalytic degradation of RhB using BiVO4/TiO2 heterostructure under visible light irradiation [J].
Hu, Yin ;
Li, Danzhen ;
Wang, Huibin ;
Zeng, Guoping ;
Li, Xionghui ;
Shao, Yu .
JOURNAL OF MOLECULAR CATALYSIS A-CHEMICAL, 2015, 408 :172-178