Research progress and challenges in hydrate-based carbon dioxide capture applications

被引:152
作者
Wang, Xiaolin [1 ]
Zhang, Fengyuan [1 ]
Lipinski, Wojciech [1 ]
机构
[1] Australian Natl Univ, Res Sch Elect Energy & Mat Engn, Canberra, ACT 2601, Australia
关键词
Hydrate-based CO2 capture; CO2 hydrate structure; Thermodynamics; Formation kinetics; PRE-COMBUSTION CAPTURE; NATURAL-GAS HYDRATE; SEMI-CLATHRATE HYDRATE; DOPED NANOPOROUS CARBONS; SEPARATION HBGS PROCESS; BUTYL AMMONIUM BROMIDE; CO2 STORAGE CAPACITY; METHANE HYDRATE; FUEL GAS; SEMICLATHRATE HYDRATE;
D O I
10.1016/j.apenergy.2020.114928
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
Climate change lends urgency to measures towards emission reduction. Carbon capture and storage is a technique that enables separation and storage of CO2 from gas mixtures before emission. Among various carbon capture methods, hydrate-based carbon capture is recognised as a promising technology due to its high CO2 storage capacity and low cost. This paper reviews recent research progress of hydrate-based carbon dioxide capture and sequestration, which is expatiated based on three stages. It discusses: (i) the influence of operating conditions on gas-water mass transfer in the mixing stage; (ii) the effects of thermodynamic promoters to tune the phase equilibrium and kinetic promoters to prompt hydrate formation and separation in the hydrate formation and capture stage; (iii) influencing factors of CH4-CO2 replacement and long-term CO2 sequestration in the sequestration stage. Further, research challenges, namely the phase equilibrium in high-pressure regions, low gas uptake and CO2 gas selectivity, contradictory experimental findings, and overlooked technical issues, are summarised. Suggestions are given for future research directions.
引用
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页数:26
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