Macaroni Fullerene Crystals-Derived Mesoporous Carbon Tubes as a High Rate Performance Supercapacitor Electrode Material

被引：40

作者：

Maji, Subrata ^{[1
]}

Shrestha, Rekha Goswami ^{[1
]}

Lee, Jaewoo ^{[2
]}

Han, Sang A. ^{[2
]}

Hill, Jonathan P. ^{[1
]}

Kim, Jung Ho ^{[2
,3
]}

Ariga, Katsuhiko ^{[1
,4
]}

Shrestha, Lok Kumar ^{[1
]}

机构：

[1] Natl Inst Mat Sci NIMS, lInt Ctr Mat Nanoarchitecton WPI MANA, 1-1 Namiki, Tsukuba, Ibaraki 3050044, Japan

[2] Univ Wollongong, Australian Inst Innovat Mat, Inst Superconducting & Elect Mat, Squires Way, North Wollongong, NSW 2500, Australia

[3] Kyung Hee Univ, Dept Adv Mat Engn Informat & Elect, 1732 Deogyeong Daero, Yongin 17104, South Korea

[4] Univ Tokyo, Grad Sch Frontier Sci, Dept Adv Mat Sci, 5-1-5 Kashiwanoha, Kashiwa, Chiba 2778561, Japan

来源：

BULLETIN OF THE CHEMICAL SOCIETY OF JAPAN | 2021年 / 94卷 / 05期

关键词：

Self-assembly; Liquid-liquid interface; Macaroni fullerene crystals; POROUS CARBON; C-60; NANOARCHITECTONICS; NANOSTRUCTURES; COMPOSITES; MICROTUBES; NANOSHEETS; NANORODS;

D O I：

10.1246/bcsj.20210059

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Self-assembled macaroni fullerene C-60 crystals (MFCs) of uniform shape and narrow size distribution are produced using the dynamic liquid-liquid interfacial precipitation method under ambient conditions. High temperature heat treatment (900 degrees C) of MFCs yields mesoporous carbons tubes (MCTs) retaining the initial morphology. This novel mesoporous carbon material exhibits excellent electrochemical supercapacitive performance due to high surface areas (1544 m(2) g(-1)), large pore volume (2.936 cm(3) g(-1)) and interconnected porous structures. In a three-electrode aqueous electrolyte system, the electrode achieved high specific capacitance ca. 422 F g(-1) at a current density of 1 A g(-1) followed by excellent cycling stability (>95%) after 10,000 charging-discharging cycles at 20 A g(-1). We believe that the novel mesoporous carbon material derived from a pi-electron carbon source can be used as an alternative electrode material in advanced supercapacitor devices.

引用

页码：1502 / 1509

页数：8

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