Photoinduced Enhancement of the Charge Density Wave Amplitude

被引:48
作者
Singer, A. [1 ]
Patel, S. K. K. [1 ,2 ]
Kukreja, R. [1 ,2 ]
Uhlir, V. [2 ]
Wingert, J. [1 ]
Festersen, S. [3 ]
Zhu, D. [4 ]
Glownia, J. M. [4 ]
Lemke, H. T. [4 ,6 ]
Nelson, S. [4 ]
Kozina, M. [4 ]
Rossnagel, K. [3 ]
Bauer, M. [3 ]
Murphy, B. M. [3 ,5 ]
Magnussen, O. M. [3 ,5 ]
Fullerton, E. E. [2 ]
Shpyrko, O. G. [1 ]
机构
[1] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA
[2] Univ Calif San Diego, Ctr Memory & Recording Res, La Jolla, CA 92093 USA
[3] Univ Kiel, Inst Expt & Appl Phys, D-24098 Kiel, Germany
[4] SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA
[5] Univ Kiel, Ruprecht Haensel Lab, D-24098 Kiel, Germany
[6] Paul Scherrer Inst, CH-5232 Villigen, Switzerland
关键词
ELECTRON; CHROMIUM; PHASE; ORDER; SUPERCONDUCTIVITY; EXCITATION; STATE;
D O I
10.1103/PhysRevLett.117.056401
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Symmetry breaking and the emergence of order is one of the most fascinating phenomena in condensed matter physics. It leads to a plethora of intriguing ground states found in antiferromagnets, Mott insulators, superconductors, and density-wave systems. Exploiting states of matter far from equilibrium can provide even more striking routes to symmetry-lowered, ordered states. Here, we demonstrate for the case of elemental chromium that moderate ultrafast photoexcitation can transiently enhance the charge-density-wave (CDW) amplitude by up to 30% above its equilibrium value, while strong excitations lead to an oscillating, large-amplitude CDW state that persists above the equilibrium transition temperature. Both effects result from dynamic electron-phonon interactions, providing an efficient mechanism to selectively transform a broad excitation of the electronic order into a well-defined, long-lived coherent lattice vibration. This mechanism may be exploited to transiently enhance order parameters in other systems with coupled degrees of freedom.
引用
收藏
页数:6
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