Nonlinear plasmonic response of doped nanowires observed by infrared nanospectroscopy

被引:14
作者
Lang, Denny [1 ,3 ]
Balaghi, Leila [1 ,2 ]
Winnerl, Stephan [1 ]
Schneider, Harald [1 ]
Huebner, Rene [1 ]
Kehr, Susanne C. [3 ]
Eng, Lukas M. [2 ,3 ]
Helm, Manfred [1 ,2 ,3 ]
Dimakis, Emmanouil [1 ]
Pashkin, Alexej [1 ]
机构
[1] Helmholtz Zentrum Dresden Rossendorf, Inst Ion Beam Phys & Mat Res, Dresden, Germany
[2] Cfaed Ctr Advancing Elect Dresden, Dresden, Germany
[3] Tech Univ Dresden, Inst Appl Phys, Dresden, Germany
关键词
s-SNIM; infrared nanospectroscopy; nanowires; free-electron laser; nonlinear plasmonics; InGaAs; GAAS NANOWIRES; TERAHERTZ; SCATTERING; SILICON; SI;
D O I
10.1088/1361-6528/aaf5a7
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
We report a strong shift of the plasma resonance in highly-doped GaAs/InGaAs core/shell nanowires (NWs) for intense infrared excitation observed by scattering-type scanning near-field infrared microscopy. The studied NWs show a sharp plasma resonance at a photon energy of about 125 meV in the case of continuous wave excitation by a CO2 laser. Probing the same NWs with the pulsed free-electron laser with peak electric field strengths up to several 10 kV cm(-1) reveals a power-dependent redshift to about 95 meV and broadening of the plasmonic resonance. We assign this effect to a substantial heating of the electrons in the conduction band and subsequent increase of the effective mass in the nonparabolic Gamma-valley.
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页数:7
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