Surface removal rate of ozone in residences in China

被引:14
作者
Yao, Mingyao [1 ]
Zhao, Bin [1 ,2 ]
机构
[1] Tsinghua Univ, Dept Bldg Sci, Sch Architecture, Beijing 100084, Peoples R China
[2] Tsinghua Univ, Beijing Key Lab Indoor Air Qual Evaluat & Control, Beijing 100084, Peoples R China
基金
中国国家自然科学基金;
关键词
Deposition velocity; Indoor air quality; Chemical reactions; Theoretical calculation; INDOOR SURFACES; DECAY-RATES; INITIATED CHEMISTRY; AIR-QUALITY; SKIN LIPIDS; PRODUCTS; TERM; POLLUTANTS; DEPOSITION; EXPOSURES;
D O I
10.1016/j.buildenv.2018.06.010
中图分类号
TU [建筑科学];
学科分类号
0813 ;
摘要
Outdoor ozone has been proven to be strongly associated with both morbidity and mortality. The deposition of ozone on indoor surfaces is the main loss of ambient ozone migrating into indoor environments, which is critical for assessing human exposure to ozone. In this study, the surface removal rate due to ozone deposition on indoor surfaces in 14 residences in China was measured. The deposition velocities for the uptake of ozone were measured as well as theoretically calculated. The results indicate that the mean standard deviation (SD) of the surface removal rate of ozone in the studied Chinese residential rooms was 2.8 +/- 1.1 h(-1). The mean SD of the measured deposition velocity was 109 +/- 34 cm/h, which is much larger than the theoretically calculated value of 27 +/- 3 cm/h. The significant difference between the measured and theoretically calculated values might result from the accumulation of organic chemicals on indoor surfaces due to the occupants' daily activities. The measured surface removal rate of ozone in Chinese residences may be further applied for estimating human exposure to ozone in China, where ozone pollution has been increasingly severe.
引用
收藏
页码:101 / 106
页数:6
相关论文
共 37 条
[1]   REMOVAL OF REACTIVE GASES AT INDOOR SURFACES - COMBINING MASS-TRANSPORT AND SURFACE KINETICS [J].
CANORUIZ, JA ;
KONG, D ;
BALAS, RB ;
NAZAROFF, WW .
ATMOSPHERIC ENVIRONMENT PART A-GENERAL TOPICS, 1993, 27 (13) :2039-2050
[2]   Assessing the Influence of Indoor Exposure to "Outdoor Ozone" on the Relationship between Ozone and Short-term Mortality in US Communities [J].
Chen, Chun ;
Zhao, Bin ;
Weschler, Charles J. .
ENVIRONMENTAL HEALTH PERSPECTIVES, 2012, 120 (02) :235-240
[3]   Ozone in indoor environments: Research progress in the past 15 years [J].
Fadeyi, Moshood Olawale .
SUSTAINABLE CITIES AND SOCIETY, 2015, 18 :78-94
[4]   Association of low-level ozone and fine particles with respiratory symptoms in children with asthma [J].
Gent, JF ;
Triche, EW ;
Holford, TR ;
Belanger, K ;
Bracken, MB ;
Beckett, WS ;
Leaderer, BP .
JAMA-JOURNAL OF THE AMERICAN MEDICAL ASSOCIATION, 2003, 290 (14) :1859-1867
[5]   Compilation of tables of surface deposition velocities for O3, NO2 and SO2 to a range of indoor surfaces [J].
Grontoft, T ;
Raychaudhuri, MR .
ATMOSPHERIC ENVIRONMENT, 2004, 38 (04) :533-544
[6]   Health-related benefits of attaining the 8-hr ozone standard [J].
Hubbell, BJ ;
Hallberg, A ;
McCubbin, DR ;
Post, E .
ENVIRONMENTAL HEALTH PERSPECTIVES, 2005, 113 (01) :73-82
[7]   Determination of ozone removal rates by selected building products using the FLEC emission cell [J].
Kleno, JG ;
Clausen, PA ;
Weschler, CJ ;
Wolkoff, P .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2001, 35 (12) :2548-2553
[8]  
Lai ACK, 2000, J AEROSOL SCI, V31, P463
[9]   Ozone decay rates in residences [J].
Lee, K ;
Vallarino, J ;
Dumyahn, T ;
Özkaynak, H ;
Spengler, JD .
JOURNAL OF THE AIR & WASTE MANAGEMENT ASSOCIATION, 1999, 49 (10) :1238-1244
[10]   Long-term ambient ozone concentration and the incidence of asthma in nonsmoking adults: The ahsmog study [J].
McDonnell, WF ;
Abbey, DE ;
Nishino, N ;
Lebowitz, MD .
ENVIRONMENTAL RESEARCH, 1999, 80 (02) :110-121