PEM Fuel Cell Catalyst Layer Structure Degradation During Carbon Corrosion

被引:3
|
作者
Borup, Rodney L. [1 ]
Mukundan, Rangachary [1 ]
Fairweather, Joseph [1 ]
Spernjak, Dusan [1 ]
Langlois, David [1 ]
Davey, John [1 ]
More, Karren [2 ]
Artyushkova, Kateryna [3 ]
机构
[1] Los Alamos Natl Lab, Los Alamos, NM 87545 USA
[2] Oak Ridge Natl Lab, Oak Ridge, TN USA
[3] Univ New Mexico, Albuquerque, NM 87131 USA
来源
POLYMER ELECTROLYTE FUEL CELLS 13 (PEFC 13) | 2013年 / 58卷 / 01期
关键词
CATHODES; SUPPORT;
D O I
10.1149/05801.0945ecst
中图分类号
O646 [电化学、电解、磁化学];
学科分类号
081704 ;
摘要
One of the major degradation involves the electrocatalyst, including the corrosion of the carbons used as catalyst supports which leads to changes in the catalyst layer structure. These changes in the catalyst layer structure lead to reduced kinetics and to mass transport limitations. The catalyst layer degradation is due to a combination of degradation mechanisms, including localized effects and depends upon operating conditions
引用
收藏
页码:945 / 952
页数:8
相关论文
共 50 条
  • [1] Automotive PEM fuel cell catalyst layer degradation mechanisms and characterisation techniques, Part I: Carbon corrosion and binder degradation
    Hegde, Sachin
    Woerner, Ralf
    Shabani, Bahman
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2025, 118 : 268 - 299
  • [2] Mitigation of PEM Fuel Cell Catalyst Degradation with Porous Carbon Supports
    Padgett, Elliot
    Yarlagadda, Venkata
    Holtz, Megan E.
    Ko, Matthew
    Levin, Barnaby D. A.
    Kukreja, Ratandeep Singh
    Ziegelbauer, Joseph M.
    Andrews, Ross N.
    Ilavsky, Jan
    Kongkanand, Anusorn
    Muller, David A.
    JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2019, 166 (04) : F198 - F207
  • [3] Understanding Catalyst Layer Degradation in PEM Fuel Cell Through Polarization Curve Fitting
    Kulikovsky, A. A.
    ELECTROCATALYSIS, 2014, 5 (03) : 221 - 225
  • [4] Understanding Catalyst Layer Degradation in PEM Fuel Cell Through Polarization Curve Fitting
    A. A. Kulikovsky
    Electrocatalysis, 2014, 5 : 221 - 225
  • [5] The Influence of Catalyst Layer Thickness on the Performance and Degradation of PEM Fuel Cell Cathodes with Constant Catalyst Loading
    Darab, Mandi
    Barnett, Alejandro Oyarce
    Lindbergh, Goran
    Thomassen, Magnus Skinlo
    Sunde, Svein
    ELECTROCHIMICA ACTA, 2017, 232 : 505 - 516
  • [6] A Simple Model for Carbon Corrosion in PEM Fuel Cell
    Kulikovsky, A. A.
    JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2011, 158 (08) : B957 - B962
  • [7] Characterization of Carbon Corrosion in a Segmented PEM Fuel Cell
    Spernjak, Dusan
    Fairweather, Joseph
    Rockward, Tommy
    Mukundan, Rangachary
    Borup, Rodney L.
    POLYMER ELECTROLYTE FUEL CELLS 11, 2011, 41 (01): : 741 - 750
  • [8] Modeling of PEM fuel cell Pt/C catalyst degradation
    Bi, Wu
    Fuller, Thomas F.
    JOURNAL OF POWER SOURCES, 2008, 178 (01) : 188 - 196
  • [9] Optimization of the PEM Fuel Cell Catalyst Layer: An Analytical Approach
    Foli, K.
    FUEL CELL SEMINAR 2009, 2010, 26 (01): : 19 - 30
  • [10] Catalyst Layer Performance in PEM Fuel Cell: Analytical Solutions
    A. A. Kulikovsky
    Electrocatalysis, 2012, 3 : 132 - 138