Dynamical screening effects of substrate phonons on two-dimensional excitons

被引:15
作者
Steinhoff, Alexander [1 ]
Florian, Matthias [1 ]
Jahnke, Frank [1 ,2 ]
机构
[1] Univ Bremen, Inst Theoret Phys, POB 330 440, D-28334 Bremen, Germany
[2] Univ Bremen, MAPEX Ctr Mat & Proc, D-28359 Bremen, Germany
关键词
LIGHT-EMITTING-DIODES; MONOLAYER; SEMICONDUCTOR; LASERS;
D O I
10.1103/PhysRevB.101.045411
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Atomically thin materials are exceedingly susceptible to their dielectric environment. For transition metal dichalcogenides, sample placement on a substrate or encapsulation in hexagonal boron nitride (hBN) are frequently used. In this paper we show that the dielectric response due to optical phonons of adjacent materials influences excitons in two-dimensional (2D) crystals. We provide an analytic model for the coupling of 2D charge carriers to optical substrate phonons, which causes polaron effects similar to that of intrinsic 2D phonons. We apply the model to hBN-encapsulated WSe2, finding a significant reduction of the exciton binding energies due to dynamical screening effects.
引用
收藏
页数:7
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共 48 条
[21]   Giant excitation induced bandgap renormalization in TMDC monolayers [J].
Meckbach, L. ;
Stroucken, T. ;
Koch, S. W. .
APPLIED PHYSICS LETTERS, 2018, 112 (06)
[22]   Influence of the effective layer thickness on the ground-state and excitonic properties of transition-metal dichalcogenide systems [J].
Meckbach, L. ;
Stroucken, T. ;
Koch, S. W. .
PHYSICAL REVIEW B, 2018, 97 (03)
[23]   Screening of a point charge by an anisotropic medium: Anamorphoses in the method of images [J].
Mele, EJ .
AMERICAN JOURNAL OF PHYSICS, 2001, 69 (05) :557-562
[24]   Ultrafast transition between exciton phases in van der Waals heterostructures [J].
Merkl, P. ;
Mooshammer, F. ;
Steinleitner, P. ;
Girnghuber, A. ;
Lin, K. -Q. ;
Nagler, P. ;
Holler, J. ;
Schueller, C. ;
Lupton, J. M. ;
Korn, T. ;
Ovesen, S. ;
Brem, S. ;
Malic, E. ;
Huber, R. .
NATURE MATERIALS, 2019, 18 (07) :691-+
[25]   Energy Spectrum of Two-Dimensional Excitons in a Nonuniform Dielectric Medium [J].
Molas, M. R. ;
Slobodeniuk, A. O. ;
Nogajewski, K. ;
Bartos, M. ;
Bala, L. ;
Babinski, A. ;
Watanabe, K. ;
Taniguchi, T. ;
Faugeras, C. ;
Potemski, M. .
PHYSICAL REVIEW LETTERS, 2019, 123 (13)
[26]   Ab Initio Calculations of Ultrashort Carrier Dynamics in Two-Dimensional Materials: Valley Depolarization in Single-Layer WSe2 [J].
Molina-Sanchez, Alejandro ;
Sangalli, Davide ;
Wirtz, Ludger ;
Marini, Andrea .
NANO LETTERS, 2017, 17 (08) :4549-4555
[27]   Temperature-dependent excitonic effects in the optical properties of single-layer MoS2 [J].
Molina-Sanchez, Alejandro ;
Palummo, Maurizia ;
Marini, Andrea ;
Wirtz, Ludger .
PHYSICAL REVIEW B, 2016, 93 (15)
[28]  
Pospischil A, 2014, NAT NANOTECHNOL, V9, P257, DOI [10.1038/NNANO.2014.14, 10.1038/nnano.2014.14]
[29]   Optical Spectrum of MoS2: Many-Body Effects and Diversity of Exciton States [J].
Qiu, Diana Y. ;
da Jornada, Felipe H. ;
Louie, Steven G. .
PHYSICAL REVIEW LETTERS, 2013, 111 (21)
[30]   Coulomb engineering of the bandgap and excitons in two-dimensional materials [J].
Raja, Archana ;
Chaves, Andrey ;
Yu, Jaeeun ;
Arefe, Ghidewon ;
Hill, Heather M. ;
Rigosi, Albert F. ;
Berkelbach, Timothy C. ;
Nagler, Philipp ;
Schueller, Christian ;
Korn, Tobias ;
Nuckolls, Colin ;
Hone, James ;
Brus, Louis E. ;
Heinz, Tony F. ;
Reichman, David R. ;
Chernikov, Alexey .
NATURE COMMUNICATIONS, 2017, 8